High-spin states and collective band structures in the odd-odd Pm-140 nucleus

The high-spin states of Pm-140 have been investigated through the reaction Te-126(F-19, 5n) at a beam energy of 90 MeV. A previous level scheme based on the 8(-) isomer has been updated with spin up to 23 (h) over bar. A total of 22 new levels and 41 new transitions were identified. Six collective bands were observed. Five of them were expanded or re-constructed, and one of them was newly identified. The systematic signature splitting and inversion of the yrast pi h(11/2)circle times vh(11/2) band in Pr and Pm odd-odd isotopes has been discussed. Based on the systematic comparison, two Delta I = 2 bands were proposed as double-decoupled bands; other two bands with strong Delta I = 1 M1 transitions inside the bands were suggested as oblate bands with gamma similar to -60 degrees; another band with large signature splitting has been proposed with oblate-triaxial deformation with gamma similar to -90 degrees. The characteristics for these bands have been discussed.

Molecular vibration spectroscopy study of irradiation effect in C-60 films induced by low energy ion

Irradiation effect in C-60 films induced by 170 keV B ion was investigated by means of Fourier transform infrared (FTIR) and Raman spectroscopies. The damage cross section sigma and the effective damage radius R are deduced from the experimental data of all four IR active modes and evident four Raman active modes of C-60 molecule. The differences on irradiation sensitivity and structural stability of the different active modes of C-60 molecule are compared. The results indicate that T-1u (4) of infrared active mode and A(g) (1) of Raman active mode are most sensitive for B ion irradiation. On the other hand T-1u (2) of infrared active mode and H-g (3) of Raman active mode are comparatively stable under B ion irradiation. (C) 2010 American Institute of Physics. [doi:10.1063/1.3512968]

Structural stability of C-60 films under the bombardment of 1.95 GeV Kr ions

The structural stability of C-60 films under the bombardment of 1.95 GeV Kr ions is investigated. The irradiated C-60 films were analyzed by Fourier Transform Infrared (FTIR) spectroscopy and Raman scattering technique. The analytical results indicate that the irradiation induced a decrease of icosahedral symmetry of C-60 molecule and damage of C-60 films; different vibration modes of C-60 molecule have different irradiation sensitivities; the mean efficient damage radius obtained from experimental data is about 1.47 nm, which is in good agreement with thermal spike model prediction.

DNA损伤检验点蛋白表达对肿瘤细胞辐射敏感性的影响

本论文应用X射线和12C6+离子对不同肿瘤细胞：HL-60、K562、SMMC-7721和HepG2进行辐照，用克隆形成率和四唑盐比色法(MTT)测定四种细胞的辐射敏感性；通过流式细胞术测定细胞周期分布、细胞凋亡、ATM和SMC1蛋白的表达变化。应用免疫细胞化学法与流式检测相结合研究了γ-H2AX蛋白表达的时间效应与剂量效应之间的关系。实验结果表明，四种细胞的辐射敏感性由强到弱依次为HL-60>K562>SMMC-7721>HepG2。即ATM表达量越低的细胞对辐射越敏感，周期阻滞水平越低，细胞凋亡越明显，但辐照后ATM蛋白的表达无显著增加，说明ATM的表达量和功能状态与细胞辐射敏感性有关，但其表达水平不能完全反映ATM蛋白激酶的活性。对ATM表达量差异最显著的HepG2和HL-60细胞来说,辐照前SMC1的表达水平与细胞S期的含量没有直接关系，辐照后SMC1蛋白的上调表达在S期阻滞修复中发挥明显的作用。辐照后1h,HL-60和HepG2细胞的H2AX磷酸化水平随吸收剂量的增加呈线性正相关,但曲线斜率与细胞辐射抗性的差异没有直接的联系。γ-H2AX的消失率与存活分数存在良好的相关性，HepG2细胞抗辐射能力强，这一时间短，HL-60细胞抗辐射能力弱，这一时间长。可以用γ-H2AX的消失速率来评估细胞的辐射敏感性。 以SMMC-7721细胞为同步化细胞模型发现，与其它同步化方法相比，步进电机旋转同步化培养法对细胞损伤最小，同步化效率最高，达到M期＞90%，GO/G1期＞80%，S期＞60%，G2/M>50%。同种射线辐照，GO/G1期SMMC-7721细胞的存活相对G2/M期来说较高。12C6+离子辐照明显减小了二者敏感度的差异性

位置灵敏塑料闪烁探测器阵列

本论文研制了一个二维位置灵敏塑料闪烁探测器阵列，该阵列由六块100 * 10 * 1 cm~3和两块100 * 5 * 1 cm~3的Pilot U型塑料闪烁体组成，所用光电管为xp2020Q型。本探测器阵列将用于重离子反应中的轻粒子角分布和飞行时间测量。本文对该种闪烁体及对应的光导中的荧光传输进行了理论计算，并用~(90)Sr-~(90)Y β源和~(252)Cf α源进行了性能测试。用~(252)Cf源的α粒子测得10cm宽的探测器的时间分辨、位置分辨和能量分辨分别为740ps、6cm和60％；测得5cm宽的探测器的分辨分别为600ps、5cm和40％。本文还介绍了用本所的MODAS-1数据获取系统对阵列进行联合测试的方法和结果，对粒子鉴别和多重性测量也进行了讨论

FEBIAD-II离子源少参数质量公式和核质量计算

第一篇FEBIAD－II离子源根据物理实验的要求本文设计和加工了一套有别于中空阴极源的FEBIAD－II离子源系统，在文中对离子源结构和特点进行了分析。测试了离子源引出离子束的发散情况，得到了此离子源的工作温度，引出离子流与高压、引出板电压、网栅电流的关系曲线，进而给出本源的工作参数。第二篇少参数质量公式和核质量计算本文介绍一个少参数的原子核质量公式，并计算了28≤Z≤81的1440个原子核质量和S_(2n)，与实验比较，核质量和S_(2n)的方均根偏差分别为1.01和0.57MeV。计算的双中子分离能曲线很好地重现了N＝50、82的主壳效应，Z＝40时N＝56的亚壳效应，以及N≥60和90时的原子核发生大形变的特性

C_(60)薄膜的荷能离子束辅照损伤效应的研究

本文简要介绍了C60的基本属性，以及荷能离子与固体相互作用的基本理论，回顾了C60辐照损伤的国内外研究现状，重点描述了在中国科学院近代物理研究所的低能离子注入机及兰州重离子加速器（HIRFL）上完成的C60薄膜的辐照实验和辐照样品的拉曼谱、X光电子谱和X射线衍射谱分析。分析结果表明荷能离子的辐照破坏了C60的分子结构和晶体结构。我们用热峰模型解释了在电子能损起主导作用能区的实验现象，分析了电子能损与核能损在C60损伤建立过程中的作用，并通过与聚合物中辐照损伤结果比较，确定了C60辐照样品中，石墨成分和无序碳成分的产生及其随辐照剂量和能损值的变化规律。在此基础上，建立了C60辐照损伤的物理图像。

板栗内皮对酸性废水中重金属的吸附

选取板栗内皮作为吸附剂,在实验室条件下,通过振荡吸附的方法研究了板栗内皮对pH 2.0的酸性废水中,镉、铅、铜、锌4种重金属离子的吸附特性。研究结果表明,当板栗内皮的加入量为30 g/L,反应时间1 h,达到对溶液中4种重金属离子的最大去除率,分别为Cd 98.9%、Pb 99.6%、Zn 98.9%、Cu 98.7%;热力学实验结果表明,板栗内皮对4种重金属离子的吸附容量分别为Cd 3.2、Pb 90.8、Zn 27.3、Cu 52.4 mg/g;动力学实验结果表明,吸附反应在60 min内可以达平衡。Elovich方程最适合描述板栗内皮吸附重金属离子的动力学行为,板栗内皮对镉、铅、铜、锌4种重金属的吸附速率和吸附时间成反比,同一时刻对4种重金属离子吸附速率大小依次是Pb2+>Cd2+>Cu2+>Zn2+。

Analysis of sulfur-containing compounds in crude oils by comprehensive two-dimensional gas chromatography with sulfur chemiluminescence detection

This paper reports an analytical method for separating, identifying, and quantifying sulfur-containing compounds in crude oil fraction (IBP-360degreesC) samples based on comprehensive two-dimensional gas chromatography coupled with a sulfur chemiluminescence detector. Various sulfur-containing compounds and their groups were analyzed with one direct injection. 3620 peaks were detected including 1722 thiols/thioethers/ disulfides/1-ring thiophenes, 953 benzothiophenes, 704 dibenzothiophenes, and 241 benzonaphthothiophenes. The target sulfur compounds and their groups were identified based on the group separation feature and structured retention of comprehensive two-dimensional gas chromatography as well as standard substances. The quantitative analysis of major sulfur-containing compounds and total sulfur was based on the linear response of the sulfur chemiluminescence detector using the internal standard method. The sulfur contents of target sulfur compounds and their groups in 4 crude oil fractions were also determined. The recoveries for standard sulfur-containing compounds were in the range of 90-102%. The quantitative result of total sulfur in the Oman crude oil fraction sample was compared with those from ASTM D 4294 standard method (total S by X-ray fluorescence spectrometry), the relative deviation (RD%) was 4.2% and the precision of the method satisfactory.

Polymeric fullerene oxide films produced by decomposition of hexanitro[60]fullerene

A new poly(fullerene oxide) thin film material has been fabricated by thermal activation and electron bombardment on hexanitro[60]fullerene (HNF) film deposited on a An substrate, all under vacuum conditions. The reaction products in the polymerization process are analyzed by XPS, UPS, IR, TGA-MS and LDI-MS techniques. It is found that the main effect of thermal and radiation treatments is to induce cleavage of -NO bonds from HNF molecules resulted in the release of nitric oxide gas and the formation of fullerene-bound oxyradicals, C-60-C-6. Spectroscopic evidence strongly suggests that rearrangement of fullerenic nitro moieties into nitrito groups is involved in the HNF decomposition process prior to the generation of reactive oxyradical intermediates. Consequently, the intermolecular coupling reaction of these oxyradicals leads to carbon polymer networks containing oxygen-bridged fullerenes. The thermally generated polymeric thin film is stable up to 900 K. Electron bombardment is also effective in both the decomposition of -NO2 groups and the removal of -OH groups present in HNF films. UV irradiation at 365 nm alone is shown to be not as efficient for the polymer formation. (C) 2003 Elsevier Ltd. All rights reserved.

长白山二道白河森林流域河岸带阔叶红松林最小面积与a多样性(英文)

河岸带是森林小流域单元的重要组成部分之一。由于河水的影响和边缘效应等因素的综合作用,河岸带植物群落与远离河岸带的森林群落在组成、结构和分布格局等方面存在较大差异,其群落最小面积也不同。本文对长白山原始阔叶红松林河岸带植物群落最小面积和物种丰富度进行了探讨。结果表明河岸带植物群落的最小面积均小于森林内部植物群落的最小面积。对于长白山原始阔叶红松林群落而言,在河岸带,包括群落的60%、80%、90%植物种类时的平均最小面积分别为80m2、180m2和320m2左右;;对应于远离河岸带的森林内部,包括群落的60%、80%、90%植物种类时的平均最小面积分别为260m2、380m2和480m2左右。河岸带植物群落的物种丰富度、均匀度和Shannon-Wiener指数普遍高于森林内部植物群落,但优势度则相反。表4参20。

长白山阔叶红松林CO_2通量季节和年际变化特征及控制机制

老龄林碳代谢的长期测定对于预测其在未来气候条件下的碳收支状态,减小陆地生态系统碳收支的不确定性十分重要．本研究使用连续两个生长季节(2003和2004年)的涡度相关CO2净交换通量测定和常规气象资料分析平均林龄200年的长白山阔叶红松林生态系统(128°28′E, 42°24′N,中国吉林省)FNEE及其主要成分FGPP与Re的季节和年际变化特征及环境和生物因子对其的影响．通量数据进行了平面坐标旋转,储存项和μ*修正．叶面积指数和温度分别控制着该生态系统FGPP和Re的季节动态和年际差别．水汽压亏缺和气温在更小尺度上调节生长季节的生态系统光合生产,根部水分条件显著影响生态系统冬季维持性的碳代谢过程．2003年1月至2004年12月该生态系统累计截获碳-449 g C·m-2,其中2003和2004年分别为-278和-171 g C·m-2．这两年FGPP和Re分别为-1332,-1294 g C·m-2和1054,1124 g C·m-2．这显示老龄森林可以成为强的碳汇．受环境因子调控,长白山阔叶红松林生态系统的碳代谢表现出显著的季节和年际差异．冬季该生态系统存在弱的光合作用,但总体上向大气释放CO2．春秋季节碳代谢非常活跃,但生态系统吸收和释放几乎相同数量的碳,对全年碳截获贡献并不显著．夏季碳代谢对该生态系统全年碳收支意义重大．90 d的夏季分别贡献全年66．9,68．9％的FGPP和60．4,62．1％的Re．

长白山阔叶红松林通量观测的footprint及源区分布

该文根据通量观测塔上2 0 0 3年12个月连续的通量观测资料,应用Schmid (1994)的FSAM(TheFlux_SourceAreaModel)模型,分析不同大气条件下源区分布.结果表明:①源(汇)区分布的基本特点是:不稳定条件下,传感器测得的通量信息源区比稳定条件时近,源区面积相对小;相同水平下非生长季的信息源区比生长季的信息源区大.②在主风方向2 0 0°～2 90°,生长季不稳定条件下,通量测量的信息源区(P =0 8)迎风方向范围在0～60 0m之间,垂直于迎风方向范围在-3 0 0～3 0 0m之间;稳定条件下,分别为0～15 0 0m ,-10 0 0～10 0 0m ;在非生长季相同大气条件下,迎风方向和垂直迎风方向的范围较均值略大些,而风向在0°～90°、90°～2 0 0°、2 90°～3 60°时,相同大气条件下,其范围与主风向生长季的范围近似.③12个月统计结果表明,76%的信息来自于西南至西北方相对均质的阔叶红松原始林,其中footprint取得最大值的源区在塔西南方10 0～40 0m范围内,几乎没有来自北偏东方向的城镇下垫面的信息,而在塔东南方0 5km以外的其他类型下垫面对通量测量的影响约3 %左右.

东北黑土土壤磷的纬向分异

以中国东北的中纬度黑土区为样带,研究了有机磷浓度与有机质、全氮浓度的关系;全磷、有机磷、无机磷及有机磷和无机磷的比率与纬度分布的关系。结果表明,有机磷和有机质、全氮浓度具有良好的相关性,它们之间的相关系数分别为0.90和0.92,呈极显著正相关(P<0.01)。全磷、有机磷、无机磷、Po/Pi在纬度上都存在不同程度的分异规律,即随着纬度的升高,其浓度或比率均有逐渐升高的趋势;其相关系数分别为0.68、0.77、0.26和0.60,相关分析表明,这些纬向分异规律都达极显著水平(P<0.01)。除了无机磷的纬向分异原因尚不明确之外,其他纬向分异的原因可能是由于黑土南北样带气候热量上的差异和人类活动的影响所致,从而造成南北样带之间有机质的矿化程度和速率产生差异。