SSC新高频腔设计与分析

Beam matching relationship between the two cyclotrons(SFC and SSC) of HIRFL is briefly discussed, and the frequency band of the new RF cavity is obtained. The new cavity is simulated with the three-dimensional electromagnetic calculation code MAFIA, and the parameters of it such as frequency, Q value, shunt impedance and voltage distribution are worked out and discussed. The simulation results show that the new RF cavity can fully meet the requirements of physics design and space configuration.中文摘要：简要分析了HIRFL SFC与SSC之间的束流匹配关系,给出了新高频腔的频率范围。利用经典三维电磁场数值模拟软件MAFIA对SSC新高频腔体进行了模拟计算,得出了SSC新高频腔体的相关物理参数,并对频率范围、Q值、并联阻抗和电压分布等参数进行了分析。高频腔体的模拟计算结果完全符合SSC回旋加速器改造的物理设计及空间结构要求。

超重复合核的存活概率

考虑角动量相关性的情况下计算了超重核259Db的裂变位垒Bf。计算了258Rf,259Db,266Hs和267Mt 4个超重核单中子蒸发的存活概率Wsur及其随角动量分波的变化关系。给出了中子蒸发宽度、裂变宽度和超重核蒸发一个中子的概率对激发能与角动量分波的依赖关系。

~(190)Tl的πh_(9/2)νi_(13/2)扁椭球转动带的旋称反转研究(英文)

利用能量为 1 6 7— 1 75MeV的35Cl束流 ,通过16 0 Gd(35Cl,5n)熔合蒸发反应研究了190 Tl的高自旋态能级结构 .实验建立了190 Tl基于πh9/2 　 　νi13/2 组态的转动带 .在束测量结果和194 Biα衰变的α γ测量结果确定地指定了190 Tl的πh9/2 　 　νi13/2 转动带的自旋值 .基于自旋指定 ,发现了190 Tl的πh9/2 　 　νi13/2 扁椭球转动带在低自旋时旋称反转 .这是首次在基于πh9/2 　 　νi13/2 组态的扁椭球转动带中观测到旋称反转 .考虑了质子 -中子剩余相互作用的粒子 -转子模型能够解释πh9/2 　 　νi13/2 扁椭球转动带的低自旋旋称反转 .

热核的衰变行为研究

中能重离子碰撞（10－100 MeV/u）为研究热核性质提供了有力的工龄。为此我们利用HIRFL提供的46.7 MeV/u ~(12)C束轰击~(159)Tb/~(197)Au/~(209)Bi研究了线动量转移分析、出平面角分布和质量分布，实验结果的分析证实了非完全熔合核的裂变和蒸发。编写了一个Monte-Carlo统计衰变程序（SAGEE）并用于详细比较C＋Au、C＋Bi的实验数据，C＋Tb的质量分布由统计两体发射理论（GEMINI）得到了解释。理论与实验的符合说明：通常类熔合反应方式形成了高激发的复合核，其后以统计两体衰变而退激。实验也统计了与裂变符合的γ能谱、三裂变的相对角度和相对速度分布，没有观察到GDR，对称三裂不是唯一的三裂方式。本文分析了HIRFL上其他小组的实验结果。研究了46.7MeV/u ~(12)C＋~(58)Ni反应的复杂粒子发射，也研究了复杂粒子出射对用放射化学方法测量的24MeV/u ~(12)C＋~(64)Cu和42MeV/u ~(12)C＋~(115)In的质量产额分布的解释。GEMINI计算很好地符合了实验结果，这意味着非完全熔合反应形成的复合核的两体衰变仍是主要的发射过程。本文也简要讨论了多重碎裂过程。基于卡西尼亚卵形体裂变形状，计算了转动核的对称和非对称形变势能，用此模型得到了核的静态裂变位垒、鞍点能并与RLDM和RFRM作了比较。我们考虑了YPE核势对核表面的弥散作用以及弥散核表面对库仑能、转动惯量的影响完善了RCOM，我们的RFCOM比RLDM和RFRM都有明显的改进，可以用于重核裂变性质研究。发展了熔合－裂变过程的宏观模型，计算了形成复合核~(149)Tb、~(194)Hg的熔合过程及其相应的裂变过程。本工作对研究热核的形成及其衰变性无疑是很有用的

Enhancement on the hydrothermal stability of ZSM-5 zeolites by the cooperation effect of exchanged lanthanum and phosphoric species

It was explored by density functional calculations that exchanged La or P species exert great influence on the local Al sites as well as on the adjacent exchanged species. In partially exchanged La- or P/H-ZSM-5 zeolite, some of the Al sites will fall off from the zeolite framework even more easily than in H-form ZSM-5, consistent with our XRF experiments. However, when exchanged by both La and P species, Al at either of the two exchanged sites shows better stability compared to H-from. zeolite. La and P species will interact strongly with each other, as evidenced by the charge donation process and the shortening of P-O-1 bond length. It was just the cooperation of La and P species that enabled RSCC catalysts worked normally under severe conditions. (C) 2004 Elsevier B.V. All rights reserved.

Characterization of the acid sites in dealuminated nanosized HZSM-5 zeolite with the probe molecule trimethylphosphine

The acid sites in dealuminated HZSM-5 zeolite with crystal sizes down to the nanoscale were firstly characterized by the probe molecule trimethylphosphine (TMP). As evidenced by the combination of P-31 CP/MAS NMR, Al-27 MAS and H-1 --> Al-27 CP/MAS NMR measurements, the Bronsted acid sites of both microsized and nanosized HZSM-5 could be decreased upon the dealumination of zeolitic framework after hydrothermal treatment. At the same time, the appearance of Lewis acid sites was observed. The dealuminated nanosized HZSM-5 is easier to form Lewis acid sites than microsized HZSM-5, and the type of Lewis acid sites in nanosized HSM-5 is more than one. In addition, the origin of Lewis acid sites is mainly associated with the aluminum at ca. 30 ppm, in the Al-27 MAS NMR spectra, and only a part of which in the dealuminated HZSM-5 zeolite acts as Lewis acid sites. (C) 2002 Elsevier Science B.V. All rights reserved.

贵州多孔菌研究Ⅰ(英文)

　对贵州省宽阔水自然保护区和黔灵山的多孔菌进行了初步研究,共发现多孔菌35种,其中中国新纪录种6个,贵州新记录种19个。3个分类单位只鉴定到属,它们明显是中国以前未报道的种类,或为新种。松生层孔菌Fomitopsispinicola(Sw :Fr )P Karst ,树舌灵芝Ganodermaapplanatum(pers.)Pat ,粗皮灵芝Ganodermatsunodae(Lloyd)Trott 和平丝硬孔菌Rigidoporuslineatus(Pers :Fr )Ryvarden为树木病原菌。