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Thanks to the courtesy of the British Museum of Natural History the author obtained from their Challenger collections two small nodules, and through a similar courtesy of the Mineralogical Department of the Riksmuseum in Stockholm one half of a much larger nodule, also from the Challenger Expedition. Results from his initial measurements of the radium contents of these samples convinced the author that the radium in the nodules is accumulated from the surrounding sediment. In the present paper the author conducted a much more thorough investigation on nodules obtained during the U.S. Albatross cruises of Dr. Agassiz. Detailed measurements of radium were conducted on individual layers and spots inside each nodule.