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During the third part of the Atlantic Expedition 1969 from 10° S to 60° N along 30° W, measurements of the complete size distribution of atmospheric aeosols over the whole size range from about 10**-7 to 10**-2 cm radius were made. This was possibe by the simultaneous operation of different methods which are critically discussed. The results obtained are the first of its kind and are of general interest despite some methodical shortcomings. North of the equator the ship passed through air masses of west African origin and the influence of Sahara dust on the Marine aerosols could be documented in a unique way. The Sahara dust component was restricted to the size range of 10**-5 to 10**-3 radius. Throughout the voyage particles up to 10**-2 radius were always found to be present, similar to findings over continents. Of special interest is the observation that the size distribution extends to very small particles, suggesting continuous aerosol production over the ocean.