巴丹吉林沙漠及其南缘地区的水化学和环境同位素特征与环境演变

The Badain Jaran Desert lies on the Alashan Plateau in western Inner Mongolia. Because of huge dunes, permanent lakes and on the northern fringe of the Asian summer monsoon, the Badain Jaran Desert has been drawing attentions of many experts. And they have made great progress in dune’s geomorphology, botany in desert, paleoclimate change and other study areas. We analyzed environmental isotope and ion chemistry in lakes and groundwater of the desert and southeastern area, and collected some other evidences from 14C dating, fossils and archeology. According to chemical analysis, we discuss the difference spatial character of ion chemistry and environmental isotope in lakes and groundwater of the desert and adjacent. Contrasting with ion chemistry and isotope results in other arid area, we argue origin of groundwater and lakes in the desert area, and get a preliminary understanding of desert lakes’ evolution during Holocene. Some main conclusions were drawn as follows: 1. It has a obvious difference in hydrophysical parameters between lakes and groundwater in the desert and margin. 2. The results of ion analysis show that Na+ and Cl- are dominant in most lakes of the desert. Meanwhile, Na+ 、Cl- and HCO3- are dominant in groundwater of the desert and adjacent, and alsoMg2+、Ca2+、and NO3- have more percentage than in lakes. 3. Owing to different solubilities, the conten of main ions in water varies with the content of TDS. Whereas the content of TDS is over 100 g/L, the content of SO42-、HCO3-、Mg2+and Ca2+ in lakes descend. 4. The result of isotope analyzing indicate the lakes and groundwater in southeast desert have a similar vaporing trend with the groundwater in the southeast margin of the desert. It imply there would have some kind of contact between groundwater in margin and lakes of southeast desert. 5. Contrasting with isotope results of groundwater in other arid area, it show that the groundwater in the desert and Yabulai area should be phreatic water which have a low water table. Therefore, we conclude that the groundwater in southeast part of the desert and southern margin mainly are recharged by precipitation of local abundant rainfall and groundwater of low mountain of southern area. 6. And all of these evidences, which are different from salinity, the content of CO32- and geological data, show that the bigger northern lake group and southeastern lake group in the desert have different groundwater replenishing system because a fold belt lie between of the two group lakes and obstruct them in landform. and HCO3- 7. The 14C dating results of fossil and lacustrine deposits show that there maybe have a wider range of shoreline during early and middle Holocene than today. 8. By the discovery and study of some pieces of pottery and fine stoneware, we preliminary conclude that there maybe have some certain amount of early human activities in the Badain Jaran Desert.

东北二龙湾玛珥湖32ka以来沉积序列的粒度组成特征及其古气候意义

Longgang maar area in Northern China is a sensitive region to the change of Asian summer monsoon, and also an important area to understand the dynamic mechanism of global paleoclimate and paleoenvironment changes. The grain-size and major element analyses have been carried out on the samples of the core from Erlongwan maar for reconstruction of high –resolution paleoenvironment change in Northeast China. Subsampling was done by 1cm interval for the upper 19.39m. Connecting multi-proxies (including,dry density, total organic carbon, etc.), we have acquired the following conclusions: 1、 the coarse fraction in grain size reflects the intensity of surface flow, and thus the intensity of monsoon rainfall in the region. 2、 the 19.39-m-long sediment covering the past 33ka, can be divided into 3 periods: The last glacial stage (33-18.5ka B.P.)：summer monsoon rainfall was low, temperature was minimum and climatic deteriorated. The last deglaciation (18.5-10 ka B.P.): temperature rose and surface water inflow increased. But it experienced a period, a Younger Dryas-like climatic deterioration. Holocene(10-0 ka B.P.)：summer monsoon rainfall reached maxima and varied at century scale and major millennial scale. 3、 the climatic variability in the whole Holocene is positively correlated with Atlantic ice-rafting events and there is an influence of sunspot activity in the late Holocene

晚中新世以来中国北方风成沉积的磁性地层学和沉积学研究

The past two decades have witnessed an unprecedented growth of interest in the palaeoenvironmental significance of the Pleistocene loess deposits in northern China. However, it is only several years ago that the Tertiary red clay sequence underlying Pleistocene loess attracted much attention. One of the major advances in recent studies of eolian deposits on the Loess Plateau is the verification of the eolian origin for the Tertiary red clay sediments. The evidence of the eolian origin for the red clay is mainly from geochemical and sedimentological studies. However, sedimentological studies of the red clay deposits are still few compared with those of the overlying loess sediments. To date, the red clay sections located near Xifeng, Baoji, Lantian, Jiaxian, and Lingtai have been studied, with an emphasis on magnetostratigraphy. These sections have a basal age ranging from ～4.3 Ma to ～7.0 Ma. The thickness of the sections varies significantly, depending perhaps on the development of local geomorphological conditions and the drainage system. Although the stratigraphy of the red clay sections has been recorded in some detail, correlation of the red clay sequences has not yet been undertaken. Geological records (Sun J. et al., 1998) have shown that during glacial periods of the Quaternary the deserts in northem China were greatly expanded compared with modern desert distribution. During interglacial periods, desert areas contracted and retreated mostly to northwestern China because of the increase in inland penetration of monsoonal precipitation. According to pedogenic characteristics of the red clay deposits, the climatic conditions of the Loess Plateau is warmer and wetter generally in the Neogene than in the late Pleistocene. Panicle analyses show that grain size distribution of the red clay sequence is similar to that of the paleosols in the Pleistocene loess record, thus implying a relatively remote provenance of the red clay materials. However, the quantitative or semiquantitative estimates of the distance from the source region to the Loess Plateau during the red clay development remains to be investigated. In this study, magnetostratigraphic and sedimentological studies are conducted at two thick red clay sequences-Jingchuan and Lingtai section. The objectives of these studies are focused on further sedimentological evidence for the eolian origin of the red clay, correlation of red clay sequences, provenance of the red clay, and the palaeoclimate reconstruction in the Neogene. Paleomagnetic studies show that the Jingchuan red clay has a basal age of 8.0 Ma, which is 1 million years older than the previously studied Lingtai section. The Lingtai red clay sequence was divided into five units on the basis of pedogenica characteristics (Ding et al., 1999a). The Jingchuan red clay sequence, however, can be lithologically divided into six units according to field observations. The upper five units of the Jingchuan red clay can generally correlate well with the five units of the Lingtai red clay. Comparison of magnetic susceptibility and color reflectance records of four red clay sections suggests that the Lingtai red clay sequence can be the type-section of the Neogene red clay deposits in northern China. Pleistocene loess and modem dust deposits have a unimodal grain-size distribution. The red clay sediments at Jingchuan and Lingtai also have a unimodal grain-size distribution especially similar to the paleosols in the Pleistocene loess record. Sedimentological studies of a north-south transect of loess deposits above S2 on the Loess Plateau show that loess deposits had distinct temporal and spatial sedimentary differentiation. The characteristics of such sedimentary differentiation can be well presented in a triangular diagram of normalized median grain size, normalized skewness, and normalized kurtosis. The triangular diagrams of the red clay-loess sequence at Lingtai and Jingchuan indicate that loess-paleosol-red clay may be transported and sorted by the same agent wind, thus extending the eolian record in the Loess Plateau from 2.6 Ma back to about 8.0 Ma. It has been recognized that during the last glacial maximum (LGM) the deserts in northern China had a distribution similar to the present, whereas during the Holocene Optimum the deserts retreated to the area west of the Helan Mountains. Advance-retreat cycles of the deserts will lead to changes in the distance of the Loess Plateau to the dust source regions, thereby controlling changes in grain size of the loess deposited in a specific site. To observe spatial changes in sedimentological characteristics of loess during the last glacial-interglacial cycle, the texture of loess was measured along the north-south transect of the Loess Plateau. Since the southern margin of the Mu Us desert during the LGM is already known, several models of grain size parameters versus the minimum distance from the source region to depositional areas were developed. According to these semiquantitative models, the minimum distance from the source region to Lingtai and Jingchuan areas is about 600 km during the Neogene. Therefore the estimated provenance of the Tertiary red clay deposits is the areas now occupied by the Badain Jaran desert and arid regions west of it. The ratio of the free iron to total iron concentration attests to being a good proxy indicator for the summer monsoon evolution. The Lingtai Fe_20_3 ratio record shows high values over three time intervals: 4.8-4.1 Ma, 3.4-2.6 Ma, and during the interglacial periods of the past 0.5 Ma. The increase in summer monsoon intensity over the three intervals also coincides with the well-developed soil characteristics. It is therefore concluded that the East-Asia summer monsoon has experienced a non-linear evolution since the late Miocene. In general, the East Asia summer monsoon was stronger in Neogene than in Quaternary and the strongest East Asia summer monsoon may occur between 4.1 and 4.8 Ma. The relatively small ice volume and high global temperature may be responsible for the strong summer monsoon during the early Pliocene.

末次盛冰期以来中国陆地生态系统碳储量变化研究

Carbon is an essential element for life, food and energy. It is also a key element in the greenhouse gases and therefore plays a vital role in climatic changes. The rapid increase in atmospheric concentration of CO_2 over the past 150 years, reaching current concentrations of about 370 ppmv, corresponds with combustion of fossii fuels since the beginning of the industrial age. Conversion of forested land to agricultural use has also redistributed carbon from plants and soils to the atmosphere. These human activities have significantly altered the global carbon cycle. Understanding the consequences of these activities in the coming decades is critical for formulating economic, energy, technology, trade, and security policies that will affect civilization for generations. Under the auspices of the International Geosphere-Biosphere Programme (IGBP), several large international scientific efforts are focused on elucidating the various aspects of the global carbon cycle of the past decade. It is only possible to balance the global carbon cycle for the 1990s if there is net carbon uptake by terrestrial ecosystems of around 2 Pg C/a. There are now some independent, direct evidences for the existence of such a sink. Policymarkers involved in the UN Framework Convention on Climate Change (UN-FCCC) are striving to reach consensuses on a 'safe path' for future emissions, the credible predictions on where and how long the terrestrial sink will either persist at its current level, or grow/decline in the future, are important to advice the policy process. The changes of terrestrial carbon storage depend not only on human activities, but also on biogeochemical and climatological processes and their interaction with the carbon cycles. In this thesis, the climate-induced changes and human-induced changes of carbon storage in China since the past 20,000 years are examined. Based on the data of the soil profiles investigated during China's Second National Soil Survey (1979-1989), the forest biomass measured during China's Fourth National Forest Resource Inventory (1989-1993), the grass biomass investigated during the First National Grassland Resource Survey (1980-1991), and the data collected from a collection of published literatures, the current terrestrial carbon storage in China is estimated to -144.1 Pg C, including -136.8 Pg C in soil and -7.3 Pg C in vegetation. The soil organic (SOC) and inorganic carbon (SIC) storage are -78.2 Pg C and -58.6 Pg C, respectively. In the vegetation reservoir, the forest carbon storage is -5.3 Pg C, and the other of-1.4 Pg C is in the grassland. Under the natural conditions, the SOC, SIC, forest and grassland carbon storage are -85.3 Pg C, -62.6 Pg C, -24.5 Pg C and -5.3 Pg C, respectively. Thus, -29.6 Pg C organic carbon has been lost due to land use with a decrease of -20.6%. At the same time, the SIC storage also has been decreased by -4.0 Pg C (-6.4%). These suggest that human activity has caused significant carbon loss in terrestrial carbon storage of China, especially in the forest ecosystem (-76% loss). Using the Paleocarbon Model (PCM) developed by Wu et al. in this paper, total terrestrial organic carbon storage in China in the Last Glacial Maximum (LGM) was -114.8 Pg C, including -23.1 Pg C in vegetation and -86.7 Pg C in soil. At the Middle Holocene (MH), the vegetation, soil and total carbon were -37.3 Pg C, -93.9 Pg C and -136.0 Pg C, respectively. This implies a gain of-21.2 Pg C in the terrestrial carbon storage from LGM to HM mainly due to the temperature increase. However, a loss of-14.4 Pg C of terrestrial organic carbon occurred in China under the current condition (before 1850) compared with the MH time, mainly due to the precipitation decrease associated with the weakening of the Asian summer monsoon. These results also suggest that the terrestrial ecosystem in China has a substantial potential in the restoration of carbon storage. This might be expected to provide an efficient way to mitigate the greenhouse warming through land management practices. Assuming that half of the carbon loss in the degraded terrestrial ecosystem in current forest and grass areas are restored during the next 50 years or so, the terrestrial ecosystem in China may sequestrate -12.0 Pg of organic carbon from the atmosphere, which represents a considerable offset to the industry's CO2 emission. If the ' Anthropocene' Era will be another climate optimum like MH due to the greenhouse effect, the sequestration would be increased again by -4.3 - 9.0 Pg C in China.

Holocene environmental changes in northeast Thailand as reconstructed from a tropical wetland

Geochemical variables (TOC, C/N, TS, delta C-13) and diatom assemblages were analyzed in a lake sediment sequence from Nong (Lake) Han Kumphawapi in northeast Thailand to reconstruct regional climatic and environmental history during the Holocene. By around c. 10,000-9400 cal yr BP, a large shallow freshwater lake had formed in the Kumphawapi basin. Oxygenated bottom waters and a well-mixed water column were characteristic of this early lake stage, which was probably initiated by higher effective moisture and a stronger summer monsoon. Decreased run-off after c. 6700 cal yr BP favored increased aquatic productivity in the shallow lake. Multiple proxies indicate a marked lowering of the lake level around 5900 cal yr BP, the development of an extensive wetland around 5400 cal yr BP, and the subsequent transition to a peatland. The shift from shallow lake to wetland and later to a peatland is interpreted as a response to lower effective moisture. A hiatus at the transition from wetland to peatland suggests very low accumulation rates, which may result from very dry climatic conditions. A rise in groundwater and lake level around 3200 cal yr BP allowed the re-establishment of a wetland in the Kumphawapi basin. However, the sediments deposited between c. 3200 and 1600 cal yr BP provide evidence for at least two hiatuses at c. 2700-2500 cal yr BP, and at c. 1900-1600 cal yr BP, which would suggest surface dryness and consequently periods of low effective moisture. Around 1600 cal yr BP a new shallow lake became re-established in the basin. Although the underlying causes for this new lake phase remain unclear, we hypothesize that higher effective moisture was the main driving force. This shallow lake phase continued up to the present but was interrupted by higher nutrient fluxes to the lake around 1000-600 cal yr BP. Whether this was caused by intensified human impact in the catchment or, whether this signals a lowering of the lake level due to reduced effective moisture, needs to be corroborated by further studies in the region. The multi-proxy study of Kumphawapi's sediment core CP3A clearly shows that Kumphawapi is a sensitive archive for recording past shifts in effective moisture, and as such in the intensity of the Asian summer monsoon. Many more continental paleorecords, however, will be needed to fully understand the spatial and temporal patterns of past changes in Asian monsoon intensity and its ecosystem impacts. (C) 2012 Elsevier B.V. All rights reserved.

Hydroclimatic shifts in northeast Thailand during the last two millennia - the record of Lake Pa Kho

The Southeast Asian mainland is located in the central path of the Asian summer monsoon, a region where paleoclimatic data are still sparse. Here we present a multi-proxy (TOC, C/N, δ¹³C, biogenic silica, and XRF elemental data) study of a 1.5m sediment/peat sequence from Lake Pa Kho, northeast Thailand, which is supported by 20 AMS ¹⁴C ages. Hydroclimatic reconstructions for Pa Kho suggest a strengthened summer monsoon between BC 170-AD 370, AD 800-960, and after AD 1450; and a weakening of the summer monsoon between AD 370-800, and AD 1300-1450. Increased run-off and a higher nutrient supply after AD 1700 can be linked to agricultural intensification and land-use changes in the region. This study fills an important gap in data coverage with respect to summer monsoon variability over Southeast Asia during the past 2000 years and enables the mean position of the Intertropical Convergence Zone (ITCZ) to be inferred based on comparisons with other regional studies. Intervals of strengthened/weaker summer monsoon rainfall suggest that the mean position of the ITCZ was located as far north as 35°N between BC 170-AD 370 and AD 800-960, whereas it likely did not reach above 17°N during the drought intervals of AD 370-800 and AD 1300-1450. The spatial pattern of rainfall variation seems to have changed after AD 1450, when the inferred moisture history for Pa Kho indicates a more southerly location of the mean position of the summer ITCZ.

Studies on the horizontal and vertical distribution of clouds and their impact on energetics of the Atmosphere over the Indian Region

Motivation for the present study is to improve the scienti c understanding on the prominent gap areas in the average three-dimensional distribution of clouds and their impact on the energetics of the earth-atmosphere system. This study is focused on the Indian subcontinent and the surrounding oceans bound within the latitude-longitude bands of 30 S to 30 N and 30 E to 110 E. Main objectives of this study are to : (i) estimate the monthly and seasonal mean vertical distributions of clouds and their spatial variations (which provide the monthly and seasonal mean 3-dimensional distributions of clouds) using multi-year satellite data and investigate their association with the general circulation of the atmosphere, (ii) investigate the characteristics of the `pool of inhibited cloudiness' that appear over the southwest Bay of Bengal during the Asian summer monsoon season (revealed by the 3-dimensional distribution of clouds) and identify the potential mechanisms for its genesis, (iii) investigate the role of SST and atmospheric thermo-dynamical parameters in regulating the vertical development and distribution of clouds, (iv) investigate the vertical distribution of tropical cirrus clouds and their descending nature using lidar observations at Thiruvananthapuram (8.5 N, 77 E), a tropical coastal station at the southwest Peninsular India, and (v) assessment of the impact of clouds on the energetics of the earth-atmosphere system, by estimating the regional seasonal mean cloud radiative forcing at top-of-the-atmosphere (TOA) and latent heating of the atmosphere by precipitating clouds using satellite data

A reconstructed Siberian High index since A. D. 1599 from Eurasian and North American tree rings

The long-term variability of the Siberian High, the dominant Northern Hemisphere anticyclone during winter, is largely unknown. To investigate how this feature varied prior to the instrumental record, we present a reconstruction of a Dec-Feb Siberian High (SH) index based on Eurasian and North American tree rings. Spanning 1599-1980, it provides information on SH variability over the past four centuries. A decline in the instrumental SH index since the late 1970s, related to Eurasian warming, is the most striking feature over the past four hundred years. It is associated with a highly significant (p < 0.0001) step change in 1989. Significant similar to 3-4 yr spectral peaks in the reconstruction fall within the range of variability of the East Asian winter monsoon (which has also declined recently) and lend further support to proposed relationships between these largescale features of the climate system.

The physical properties of the atmosphere in the new Hadley Centre Global Environmental Model (HadGEM1). Part II: Aspects of variability and regional climate

The performance of the atmospheric component of the new Hadley Centre Global Environmental Model (HadGEM1) is assessed in terms of its ability to represent a selection of key aspects of variability in the Tropics and extratropics. These include midlatitude storm tracks and blocking activity, synoptic variability over Europe, and the North Atlantic Oscillation together with tropical convection, the Madden-Julian oscillation, and the Asian summer monsoon. Comparisons with the previous model, the Third Hadley Centre Coupled Ocean-Atmosphere GCM (HadCM3), demonstrate that there has been a considerable increase in the transient eddy kinetic energy (EKE), bringing HadGEM1 into closer agreement with current reanalyses. This increase in EKE results from the increased horizontal resolution and, in combination with the improved physical parameterizations, leads to improvements in the representation of Northern Hemisphere storm tracks and blocking. The simulation of synoptic weather regimes over Europe is also greatly improved compared to HadCM3, again due to both increased resolution and other model developments. The variability of convection in the equatorial region is generally stronger and closer to observations than in HadCM3. There is, however, still limited convective variance coincident with several of the observed equatorial wave modes. Simulation of the Madden-Julian oscillation is improved in HadGEM1: both the activity and interannual variability are increased and the eastward propagation, although slower than observed, is much better simulated. While some aspects of the climatology of the Asian summer monsoon are improved in HadGEM1, the upper-level winds are too weak and the simulation of precipitation deteriorates. The dominant modes of monsoon interannual variability are similar in the two models, although in HadCM3 this is linked to SST forcing, while in HadGEM1 internal variability dominates. Overall, analysis of the phenomena considered here indicates that HadGEM1 performs well and, in many important respects, improves upon HadCM3. Together with the improved representation of the mean climate, this improvement in the simulation of atmospheric variability suggests that HadGEM1 provides a sound basis for future studies of climate and climate change.

ENSO at 6ka and 21ka from ocean–atmosphere coupled model simulations

We analyze how the characteristics of El Niño-Southern Oscillation (ENSO) are changed in coupled ocean–atmosphere simulations of the mid-Holocene (MH) and the Last Glacial Maximum (LGM) performed as part of the Paleoclimate Modeling Intercomparison Project phase 2 (PMIP2). Comparison of the model results with present day observations show that most of the models reproduce the large scale features of the tropical Pacific like the SST gradient, the mean SST and the mean seasonal cycles. All models simulate the ENSO variability, although with different skill. Our analyses show that several relationships between El Niño amplitude and the mean state across the different control simulations are still valid for simulations of the MH and the LGM. Results for the MH show a consistent El Niño amplitude decrease. It can be related to the large scale atmospheric circulation changes. While the Northern Hemisphere receives more insolation during the summer time, the Asian summer monsoon system is strengthened which leads to the enhancement of the Walker circulation. Easterlies prevailing over the central eastern Pacific induce an equatorial upwelling that damps the El Niño development. Results are less conclusive for 21ka. Large scale dynamic competes with changes in local heat fluxes, so that model shows a wide range of responses, as it is the case in future climate projections.

Arctic Oscillation and Antarctic Oscillation in internal atmospheric variability

n this study, we investigated the features of Arctic Oscillation (AO) and Antarctic Oscillation (AAO), that is, the annular modes in the extratropics, in the internal atmospheric variability attained through an ensemble of integrations by an atmospheric general circulation model (AGCM) forced with the global observed SSTs. We focused on the interannual variability of AO/AAO, which is dominated by internal atmospheric variability. In comparison with previous observed results, the AO/AAO in internal atmospheric variability bear some similar characteristics, but exhibit a much clearer spatial structure: significant correlation between the North Pacific and North Atlantic centers of action, much stronger and more significant associated precipitation anomalies, and the meridional displacement of upper-tropospheric westerly jet streams in the Northern/Southern Hemisphere. In addition, we examined the relationship between the North Atlantic Oscillation (NAO)/AO and East Asian winter monsoon (EAWM). It has been shown that in the internal atmospheric variability, the EAWM variation is significantly related to the NAO through upper-tropospheric atmospheric teleconnection patterns.

Climatology of polar lows over the Sea of Japan using the JRA-55 reanalysis

Polar lows are intense meso- a -scale cyclones that develop over the oceans poleward of the main baroclinic zone. A number of previous studies have reported polar low formation over the Sea of Japan within the East Asian winter monsoon. To understand the climatology of polar lows over the Sea of Japan, a tracking al- gorithm for polar lows is applied to the recent JRA-55 reanalysis. The polar low tracking is applied to 36 cold seasons (October–March) from October 1979 to March 2015. The polar lows over the Sea of Japan reach their maximum intensity on the southeastern side of the midline between the Japanese islands and the Asian continent. Consistent with previous case studies, composite analysis demonstrates that the polar low devel- opment is associated with the enhanced northerly flow on the western side of a synoptic-scale extratropical cyclone, with the cold trough in the midtroposphere and with increased heat fluxes from the sea surface. Furthermore, the present climatological study has revealed two dominant directions of motion of the polar lows: southward and eastward. Southward-moving polar lows are steered by a strong northerly flow in the lower troposphere, which is enhanced on the western side of synoptic-scale extratropical cyclones, while the eastward-moving polar lows occur within a planetary-scale westerly flow in the midlatitudes. Thus, the di- rection of polar low motion reflects the difference in planetary- and synoptic-scale conditions.

Untersuchung von Mischungs- und Transportprozessen in der oberen Troposphäre - unteren Stratosphäre basierend auf in-situ Spurengasmessungen

Die obere Troposphäre / untere Stratosphäre (UTLS: Upper Troposphere / Lower Stratosphere)ist die Übergangsgregion zwischen den dynamisch, chemisch und mikrophysikalisch sehr verschiedenen untersten Atmosphärenschichten, der Troposphäre und der Stratosphäre. Strahlungsaktive Spurengase, wie zum Beispiel Wasserdampf (H2O), Ozon (O3) oder Kohlenstoffdioxid (CO2), und Wolken in der UTLS beeinflussen das Strahlungsbudget der Atmosphäre und das globale Klima. Mögliche Veränderungen in den Verteilungen und Konzentrationen dieser Spurengase modifizieren den Strahlungsantrieb der Atmosphäre und können zum beobachteten Klimawandel beitragen. Ziel dieser Arbeit ist es, Austausch- und Mischungsprozesse innerhalb der UTLS besser zu verstehen und damit Veränderungen der Spurengaszusammensetzung dieser Region genauer prognostizieren zu können. Grundlage hierfür bilden flugzeuggetragene in-situ Spurengasmessungen in der UTLS, welche während der Flugzeugmesskampagnen TACTS / ESMVal 2012 und AIRTOSS - ICE 2013 durchgeführt wurden. Hierbei wurde bei den Messungen von AIRTOSS - ICE 2013 das im Rahmen dieser Arbeit aufgebaute UMAQS (University of Mainz Airborne QCLbased Spectrometer) - Instrument zur Messung der troposphärischen Spurengase Distickstoffmonoxid (N2O) und Kohlenstoffmonoxid (CO) eingesetzt. Dieses erreicht bei einer zeitlichen Auflösung von 1 s eine Messunsicherheit von 0,39 ppbv und 1,39 ppbv der N2O bzw. CO-Mischungsverhältnisse. Die hohe Zeitauflösung und Messgenauigkeit der N2O- und CO- Daten erlaubt die Untersuchung von kleinskaligen Austauschprozessen zwischen Troposphäre und Stratosphäre im Bereich der Tropopause auf räumlichen Skalen kleiner 200 m. Anhand der N2O-Daten von AIRTOSS - ICE 2013 können in-situ detektierte Zirruspartikel in eisübersättigter Luft oberhalb der N2O-basierten chemischen Tropopause nachgewiesen werden. Mit Hilfe der N2O-CO-Korrelation sowie der Analyse von ECMWF-Modelldaten und der Berechnung von Rückwärtstrajektorien kann deren Existenz auf das irreversible Vermischen von troposphärischen und stratosphärischen Luftmassen zurückgeführt werden. Mit den in-situ Messungen von N2O, CO und CH4 (Methan) von TACTS und ESMVal 2012 werden die großräumigen Spurengasverteilungen bis zu einer potentiellen Temperatur von Theta = 410 K in der extratropischen Stratosphäre untersucht. Hierbei kann eine Verjüngung der Luftmassen in der extratropischen Stratosphäre mit Delta Theta > 30 K (relativ zur dynamischen Tropopause) über den Zeitraum der Messkampagne (28.08.2012 - 27.09.2012) nachgewiesen werden. Die Korrelation von N2O mit O3 zeigt, dass diese Verjüngung aufgrund des verstärkten Eintrages von Luftmassen aus der tropischen unteren Stratosphäre verursacht wird. Diese werden über den flachen Zweig der Brewer-Dobson-Zirkulation auf Zeitskalen von wenigen Wochen in die extratropische Stratosphäre transportiert. Anhandrnder Analyse der CO-O3-Korrelation eines Messfluges vom 30.08.2012 wird das irreversible Einmischen von Luftmassen aus der tropischen Stratosphäre in die Extratropen auf Isentropen mit Theta > 380 K identifiziert. Rückwärtstrajektorien zeigen, dass der Ursprung der eingemischten tropischen Luftmassen im Bereich der sommerlichen Antizyklone des asiatischen Monsuns liegt.

Precipitation over the past four centuries in the Dieshan Mountains as inferred from tree rings: An introduction to an HHT-based method

To improve our understanding of the Asian monsoon system, we developed a hydroclimate reconstruction in a marginal monsoon shoulder region for the period prior to the industrial era. Here, we present the first moisture sensitive tree-ring chronology, spanning 501 years for the Dieshan Mountain area, a boundary region of the Asian summer monsoon in the northeastern Tibetan Plateau. This reconstruction was derived from 101 cores of 68 old-growth Chinese pine (Pinus tabulaeformis) trees. We introduce a Hilbert–Huang Transform (HHT) based standardization method to develop the tree-ring chronology, which has the advantages of excluding non-climatic disturbances in individual tree-ring series. Based on the reliable portion of the chronology, we reconstructed the annual (prior July to current June) precipitation history since 1637 for the Dieshan Mountain area and were able to explain 41.3% of the variance. The extremely dry years in this reconstruction were also found in historical documents and are also associated with El Niño episodes. Dry periods were reconstructed for 1718–1725, 1766–1770 and 1920–1933, whereas 1782–1788 and 1979–1985 were wet periods. The spatial signatures of these events were supported by data from other marginal regions of the Asian summer monsoon. Over the past four centuries, out-of-phase relationships between hydroclimate variations in the Dieshan Mountain area and far western Mongolia were observed during the 1718–1725 and 1766–1770 dry periods and the 1979–1985 wet period.

Age models of ODP Site 184-1143

Here we present an improved astronomical timescale since 5 Ma as recorded in the ODP Site 1143 in the southern South China Sea, using a recently published Asian summer monsoon record (hematite to goethite content ratio, Hm/Gt) and a parallel benthic d18O record. Correlation of the benthic d18O record to the stack of 57 globally distributed benthic d18O records (LR04 stack) and the Hm/Gt curve to the 65°N summer insolation curve is a particularly useful approach to obtain refined timescales. Hence, it constitutes the basis for our effort. Our proposed modifications result in a more accurate and robust chronology than the existing astronomical timescale for the ODP Site 1143. This updated timescale further enables a detailed study of the orbital variability of low-latitude Asian summer monsoon throughout the Plio-Pleistocene. Comparison of the Hm/Gt record with the d18O record from the same core reveals that the oscillations of low-latitude Asian summer monsoon over orbital scales differed considerably from the glacial-interglacial climate cycles. The popular view that summer monsoon intensifies during interglacial stages and weakens during glacial stages appears to be too simplistic for low-latitude Asia. In low-latitude Asia, some strong summer monsoon intervals appear to have also occurred during glacial stages in addition to their increased occurrence during interglacial stages. Vice versa, some notably weak summer monsoon intervals have also occurred during interglacial stages next to their anticipated occurrence during glacial stages. The well-known mid-Pleistocene transition (MPT) is only identified in the benthic d18O record but not in the Hm/Gt record from the same core. This suggests that the MPT may be a feature of high- and middle-latitude climates, possibly determined by high-latitude ice sheet dynamics. For low-latitude monsoonal climate, its orbital-scale variations respond more directly to insolation and are little influenced by high-latitude processes, thus the MPT is likely not recorded. In addition, the Hm/Gt record suggests that low-latitude Asian summer monsoon intensity has a long-term decreasing trend since 2.8 Ma with increased oscillation amplitude. This long-term variability is presumably linked to the Northern Hemisphere glaciation since then.