短寿命缺中子同位素~(130,129,128)Ce的(EC+β~+)衰变

首次报道130Ce、129Ce和128Ce的(EC+β+)衰变纲图,其中包括核素的产生、核素的分离鉴别以及纲图的建立。着重补充了一些重要的技术细节,更新了129Ce的衰变纲图,并对这些纲图中涉及的物理问题进行了讨论。

进一步指认近质子滴线核~(129)Pm的衰变

20 0 4年曾报道过利用4 0 Ca + 92 Mo融合蒸发反应产生了近质子滴线新核素12 9Pm ,并首次观测到它 (EC + β+)衰变产生的能量为 99keV的γ射线 .为了进一步确认上述指认 ,以下提供了三方面的新证据 :1)在 16 4— 190MeV能量范围内测量了 99keV衰变γ射线的激发函数 ;2 )进行了交叉反应36 Ar + 96 Ru的实验 ,观察到了相同的 99keV衰变γ射线 ;3)用Woods SaxonStrutinsky方法计算了12 9Pm的核势能面 ,其基态自旋宇称被预言为 5 / 2 - ,所以12 9Pm的 (EC + β+)衰变有利于馈送到子核12 9Nd的 5 / 2 - 的低位态 ,这也与前期报道相符 .

Assessment of I-129 measurement at low MV tandem voltages

IEECAS SKLLQG

~(129)Xe~(30+)轰击Ni表面激发靶原子偶极跃迁和禁戒(M1和E2)跃迁的特征光谱线

报道了用高电荷态离子1 2 9Xe30 + (15 0keV)轰击金属Ni表面 ,激发的 2 0 0— 10 0 0nmNiⅠ和NiⅡ的特征光谱线的实验结果 .实验结果表明 :用电荷态足够高的离子作光谱激发源 ,无需很强的束流强度 (nA量级 ) ,便可有效地产生原子和离子的复杂组态间跃迁所形成的可见光波段的特征谱线 ,特别是NiⅠ和NiⅡ偶极禁戒的电四极跃迁E2和磁偶极跃迁M1的特征光谱线 .通过分析发现 ,在禁戒跃迁的谱线中 ,有些是电子组态相同而原子态不同的偶极禁戒跃迁光谱线而且NiⅡ的 6 84 84nm谱线较强

质子滴线附近的新核素~(129)Pm

通过重离子引起的融合蒸发反应 92 Mo (40 Ca ,p2n)合成了稀土区未知核素 12 9Pm ,并且配合氦喷嘴快速带传输系统利用X γ符合方法对它进行了首次鉴别 .实验观测到了经 12 9Pm的 (EC +β+ )衰变产生的对应于子核 12 9Nd中 5 2 -→ 1 2 -跃迁的一条 99keVγ线 .根据这条 99keVγ线的时间衰变曲线 ,提取出 12 9Pm的半衰期为 (2 .4± 0 .6 )s .

缺中子核素~(129)Ce的(EC/β~+)衰变

利用 10 2MeV16O6+束轰击同位素靶117Sn ,通过熔合蒸发 4n反应产生核素12 9Ce.由氦喷嘴快速带传输系统将反应产物送到低本底区 .通过化学分离来制备待测的Ce样品 ,与此同时用16O束轰击117Sn的两种相邻的同位素靶118Sn和116Sn ,并比较上述 3种反应中的产物来进一步区分元素Ce的不同的同位素 .结果一种半衰期为 4.1min的活性被鉴定为12 9Ce.基于X -γ -t和γ -γ -t符合测量 ,建议了包括 5 1条射线在内的12 9Ce的 (EC/ β+)衰变纲图 .其中 ,12 9Ce基态直接馈送到12 9La基态的份额 ( 2 6± 7) %是用观测到的12 9La衰变的 2 78.6keV的γ射线的生长和衰变曲线估计出来的 .另外还给出了用La Kα X射线和6 8.2keVγ射线开门的γ谱以及典型的衰变γ射线的时间谱

X-ray spectra induced by Xe-129(q+) impacting the metal surface

Using the slow highly charged ions Xe-129(q+) (q = 25, 26, 27; initial kinetic T-0 <= 4.65 keV/a.u.) to impact Au surface, the Au atomic M alpha characteristic X-ray spectrum is induced. The result shows that as long as the charge state of projectile is high enough, the heavy atomic characteristic X-ray can be effectively excited even though the incident beam is very weak (nA magnitude), and the X-ray yield per ion is in the order of 10(-8) and increases with the kinetic energy and potential energy of projectile. By measuring the Au M alpha-X-ray spectra, Au atomic N-level lifetime is estimated at about 1.33x10(-18) s based on Heisenberg uncertainty relation.

2.6 s isomer of Nd-129

Nd-129 was produced by irradiation of an enriched target of Ru-96 with a Ar-36 beam and studied by using a helium-jet fast tape transport system in combination with X-gamma and gamma-gamma coincidence measurements. A 2.6s isomer of Nd-129 was observed for the first time and tentatively proposed to be the configuration of 1/2[411].

X-ray spectrum emitted by the impact of Xe-129(q+) on Mo surface

We studied the characteristic X-ray spectra produced by the interaction of highly charged ions of X-129(q+) (q =25, 26, 27) with surface of metallic Mo. The experimental result shows that highly charged ions can excite the characteristic X-ray spectra of L-shell of Mo when the beam' s intensity is not more than 120 nA. The X-ray yield of single ion reaches a quantitative level of 10(-8) and increases with the increment of the ion' s kinetic energy and ionic charge (potential energy). By measuring the X-ray spectra of Mo-L alpha(1) the M-level lifetime of Mo atom is estimated by using Heisenberg uncertainty relation.

~(129)Xe~(q+)激发Mo表面产生的X射线谱；X-ray spectrum emitted by the impact of ~(129)Xe~(q+) on Mo surface

研究了高电荷态离子129Xeq+(q=25,26,27)入射金属Mo表面产生的特征X射线谱.实验结果表明,在束流强度小于120nA条件下,高电荷态离子129Xeq+可以激发Mo的L壳层特征X射线谱.单离子X射线相对产额可达10-8量级,特征X射线的相对产额随入射离子的动能和电荷态(势能)的增加而增加.通过Mo原子的Lα1特征X射线谱,利用Heisenberg不确定关系对Mo原子的第M能级寿命进行了估算.

THE TRANSFER OF METAL-IONS ACROSS THE WATER-NITROBENZENE INTERFACE FACILITATED BY NEUTRAL CARRIER ETH-129

The transfer of H+, Li+, Na+, Zn2+, Mg2+ and Cu2+ facilitated by ionophore ETH 129 (N, N, N', N'-tetracyolohexyl-3-oxapentanediamide) across water/nitrobenzene interface has been studied by the cyclic voltammetry. The mechanism of the transfer process has been discussed. The diffusion coefficients and the stability constants of the complexes formed in the nitrobenzene phase have been determined.