987 resultados para Ar - Poluição


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利用硅半导体+CsI(T1)闪烁体望远镜测量35MeV/u40Ar+197Au中发射的轻带电粒子,用能谱斜率方法和双同位素产额比方法提取了核温度参量.研究了热核发射过程中的统计发射规律.

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测量了 3 0MeV/u40 Ar束流轰击115 In反应靶时出射的中等质量碎片(IMF)的能谱 .通过比较在不同出射角度发射的同一种IMF的能谱 ,得到了IMF的发射机制随出射角的演化关系 .在假定运动源速度和出射离子库仑位垒不随出射角变化的条件下 ,通过改变发射源的强度和核温度参量完成了对实验测得能谱的运动源拟合 ,并详细讨论了 3个发射源所占份额和源强随出射角的演化关系 .

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采用紫外 -可见光吸收技术分析和研究了 35MeV/uAr离子辐照聚酯膜引起的光吸收改性 .结果表明 ,Ar离子轰击聚酯膜时引起了碳键的共轭体系形成 ,从而导致了紫外 -可见光区域中光吸收明显增加 ,光吸收增加的幅度依赖于离子的照射剂量、离子在样品中的平均电子能量损失以及光的波长 ,剂量越高 ,电子能损越大 ,光吸收增幅越大 ;而光的波长越长 ,光吸收的增加则越不明显 .利用测量到的光吸收曲线 ,同时还定量地研究了各种辐照条件下聚酯膜的光能隙和碳原子团的尺寸 .

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从 2 5MeV/u4 0 Ar+115In反应前中角区出射碎片的能谱、角分布和Z电荷分布出发 ,讨论了碎片发射机制随出射角和核电荷数Z的渐进变化 ;用改进的量子分子动力学 (MQMD)模型研究了碎片角分布及Z电荷分布 ,理论计算和实验值整体上符合较好 ,但在前角区MQMD模型低估了碎片的产额 ,在中角区对于Z接近弹核的碎片 ,理论计算比实验值偏高 ;碎片产物的角分布及Z电荷分布还与统计模型GEMINI进行了比较 ,发现在前角区平衡蒸发的成分所占比例很小 ,中角区所占的比例有所增加 ,但仍然是较小的比例 .随着碎片核电荷数Z的减小 ,平衡核的蒸发成分逐渐减少 ,非平衡的中速成分逐渐占主导地位

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35MeV/u Ar离子在室温下辐照了多层堆叠的半晶质聚酯膜,采用傅立叶转换的红外光吸收技术分析和研究了由辐照引起的化学键断裂及其对离子剂量、离子在样品中的平均电子能量损失和吸收剂量的依赖性.结果表明,辐照导致聚酯膜中发生了明显的化学键断裂,断键过程主要发生在反式构型的乙二醇残留物和苯环的对位上,苯环的基本结构在辐照中变化较小.断键不仅强烈地依赖于离子的照射剂量,而且还跟样品中电子能量沉积密切相关,明显的断键发生在4.0MGy以上的吸收剂量.

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报道了 30MeV/ u(40)Ar+(nat)Ag反应中中等质量碎片(IMF)发射时间(τ)随发射源空间大小的演化规律,并对类弹碎片的发射时空进行了讨论.结果表明,IMF的发射时标与中等质量碎片关联函数以及发射源的核物质密度(ρ)有关,而与发射源的质量数的关系不大.对于能量较高的类弹碎片来说,在较小的核物质密度下提取的发射时间也较小,因此,在正常核物质密度参数下提取出的发射时间值可作为碎片实际发射时间的上限值.中速碎片的发射时间随密度大小的变化非常缓慢,提取出的发射时间值即可作为实际的发射时间。

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测量了 25MeV/u40 Ar+115 In,58 Ni,27 A1反应前中角区出射碎片的角分布和 元素 Z分布.用改进的量子分子动力学(MQMD)模型研究了碎片的角分布和 Z 分布.理论计算值和实验值整体上符合得很好,但在前角区,MQMD模型低估 了碎片的产额,在中角区对于Z接近弹核的碎片,理论计算值比实验值偏高.碎 片产物的角分布和Z分布还与统计蒸发模型GEMINI进行了比较,结果表明,在 前角区平衡蒸发成份所占的比例很小,中角区所占的比例有所增加,但仍然是较 小的比例.同时发现平衡蒸发成份随着出射碎片核电荷数Z的减小而逐渐减 少.

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Size modification of Au nanoparticles (NPs), deposited on the Au-thick film surface and irradiated by slow highly charged ions (SHCI) 40Arq+ (3 6 q 6 12) with fixed low dose of 4.3 1011 ions/cm2 and various energy ranging from 74.64 to 290.64 keV at room temperature (293.15 K), was investigated by atomic force microscopy (AFM) and transmission electron microscopy (TEM). The effect of projectile kinetic energy on the modified size of NPs was explored by an appropriate choice of the fixed process parameters such as ion flux, irradiation temperature, incident angle, irradiation time, etc. The morphological changes of NPs were interpreted by models involving collisional mixing, Ostwald ripening (OR) and inverse Ostwald ripening (IOR) of spherical NPs on a substrate. A critical kinetic energy as well as a critical potential energy of the projectile in the Au NPs size modification process were observed.

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The ratios R-k1 of k-fold to single ionization of the target atom with simultaneous one-electron capture by the projectile have been measured for 15-480 keV/u (nu(p) = 0.8-4.4 a.u.) collisions of Cq+, Oq+ (q=1-4) with Ar, using time-of-flight techniques which allowed the simultaneous identification of the final charge state of both the low-velocity recoil ion and the high-velocity projectile for each collision event. The present ratios are similar to those for He+ and He2+ ion impact. The energy dependence of R-k1 shows a maximum at a certain energy, E-max. which approximately conforms to the q(1/2)-dependence scaling. For a fixed projectile state, the ratios R-k1 also vary strongly with outgoing reaction channels. The general behavior of the measured data can be qualitatively analyzed by a simple impact-parameter, independent-electron model. (C) 2009 Elsevier B.V. All rights reserved.

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The highly charged ion Ar-40(16+) with the velocity (kinetic energy E (K)=150 keV, velocity V=8.5x10(5) m/s) smaller than Bohr velocity (V (Bohr)=2.9x10(6) m/s) was found to hove impacts on the surfaces of metals Ni, Mo, Au and Al, and the Ar atomic infrared light lines and X-rays spectra were simultaneously measured. The experimental results show that the highly charged ion that captures electrons is neutralized, and the multiply-excited hollow atom forms. The hollow atom cascade decay radiates lights from infrared to X-ray spectrum. The intensity of infrared lights shows that the metallic work functions play an important role in the neutralization process of highly charged ions during their interaction with metallic surfaces, which verifies the classical over-the-barrier model.

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对注入Ar+后不同晶面取向的蓝宝石晶体在不同退火条件下的光致发光谱进行了分析.分析结果表明:三种晶面取向的蓝宝石样品经Ar+注入后,其光致发光谱中均出现了新的位于506nm处的发光峰;真空和空气气氛下的退火均对样品在506nm处的发光有增强作用,不同晶面取向的样品发光增强程度不同,且发光增强至最大时的退火温度也不同,空气气氛下的退火使样品发光增强程度更为显著.由此可以看出,退火气氛、退火温度和晶面取向均对样品发光峰强度有影响.

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The reduced velocity correlation functions of the Intermediate Mass Fragments (IMFs) were measured in the reactions of Ar-36+ Sn-112,Sn-124 at 35MeV/u. The anti-correlation at small reduced velocities is more pronounced in Ar-36+ Sn-124 system than that in Ar-36+ Sn-112 system. The difference of the correlation functions between the two reactions is mainly contributed by the particle pairs with high momenta. A three-body Coulomb repulsive trajectory code (MENEKA) is employed to calculate the emission time scale of IMFs for-the both systems. The time scale is 150fm/c in the Ar-36+ Sn-112 system and 120fm/c in the Ar-36+ Sn-124 system, respectively. A calculation based on an Isospin dependence Quantum Molecular Dynamics code (IQMD) reveals that the emission time spectrum of IMFs is shifted slightly leftwards in Ar-36+ Sn-124 compared with that in the Ar-16+ Sn-112 system, indicating a shorter emission time scale. Correspondingly, the central density of the hot nuclei decreases faster in Ar-36+ Sn-124 than in Ar-36+ Sn-112

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Employing the recoil ion momentum spectroscopy we investigate the collision between He2+ and argon atoms. By measuring the recoil longitudinal momentum the energy losses of projectile are deduced for capture reaction channels. It is found that in most cases for single- and double-electron capture, the inner electron in the target atom is removed, the recoil ion is in singly or multiply excited states (hollow ion is formed), which indicates that electron correlation plays an important role in the process. The captured electrons prefer the ground states of the projectile. It is experimentally demonstrated that the average energy losses are directly related to charge transfer and electronic configuration.

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By use of optical spectrum technology, the spectra of X-ray induced by highly charged Ar-40(q+) ions interacting with Au surface have been studied. The results show that the argon K alpha X-ray were emitted from the hollow atoms formed below the surface. There is a process of multi-electron exciting in neutralization of the Ar16+ ion, with electronic configuration 1s(2) in its ground state below the solid surface. The yield of the projectile K alpha X-ray is related to its initial electronic configuration, and the yield of the target X-ray is related to the projectile kinetic energy.

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用速度不同的(动能EK=272和357keV,速度v=1.14×106和1.72×106m/s)的高电荷态离子40Ar17+分别入射金属Be表面,同时测量这种相互作用过程中产生的近红外光谱线和X射线谱。实验结果表明,在低速范围内(速度小于玻尔速度vBohr=2.19×106m/s),速度较小的40Ar17+离子在到达金属的表面临界距离Rc到进入表面(2—3原子层)的进程中,形成了较多的高激发态Ar原子,其退激辐射较强的光谱线,进而验证了经典过垒模型。