24 resultados para Síntese granular
Resumo:
CoFe-AgCu granular films of compositions ranging from 0.17-0.44 ferromagnetic atomic concentration were prepared by rf sputtering. The microstructure and the transport and magnetic properties suggested that this family of samples can be classified into two groups with a crossover concentration at about 32 at. %. The experimental results for samples Co34Fe8Ag54Cu4 and Co18Fe8Ag70Cu4, which are representative of both different behaviors, are discussed. For the as-prepared sample with higher CoFe content, an uncompensated out-of-plane antiferromagneticlike microstructure with dominant demagnetizing interactions was observed. The particle growth through the annealing led to large in-plane ferromagneticlike clusters with dominant magnetizing interactions. The thermal dependence of the remanence-to-saturation ratio of the as-prepared and annealed samples indicated the existence of a high degree of magnetic correlations leading to a very low magnetoresistivity: In none of the cases was a Stoner¿Wohlfarth behavior observed. On the contrary, for the sample with lower CoFe content, the magnetoresistivity change was much higher, and the remanence followed the expected behavior, since magnetic correlations were strongly reduced through dilution.
Resumo:
The ac electrical response is studied in thin films composed of well-defined nanometric Co particles embedded in an insulating ZrO2 matrix which tends to coat them, preventing the formation of aggregates. In the dielectric regime, ac transport originates from the competition between interparticle capacitive Cp and tunneling Rt channels, the latter being thermally assisted. This competition yields an absorption phenomenon at a characteristic frequency 1/(RtCp), which is observed in the range 1010 000 Hz. In this way, the effective ac properties mimic the universal response of disordered dielectric materials. Temperature and frequency determine the complexity and nature of the ac electrical paths, which have been successfully modeled by an Rt-Cp network.
Resumo:
We have observed a type of giant magnetoresistance (GMR) in magnetic granular Co10Cu90 alloys. The asymmetric GMR depends strongly on the size of magnetic Co particles, which exhibit superparamagnetic behavior at given measured temperature. The asymmetric GMR points to a metastable state that develops when the sample is field-cooled, which is lost after recycling. We propose that high-field cooling produces more effective parallel alignment of small unblocked Co particle moments and interfacial magnetizations, which contributes to the further decrease of the resistance in comparison with the samples zero-field-cooled, and then applied to the same field.
Resumo:
El concepto de aspereza equivalente (ks) permite relacionar la resistencia al flujo de cauces de contorno granular con el tamaño de las partículas que lo conforman, mediante la ley logarítmica de distribución vertical de velocidad de la corriente. En este artículo se revisa el estado del conocimiento acerca de los criterios para la predicción de dicha relación con el objetivo de brindar una guía para la selección de los mismos. Pese a que el análisis de las experiencias compiladas desvela la dispersión de resultados, a efectos prácticos se recomienda para ríos de grava y de montaña: ks 3•d90; ks 3,4•d84 y ks 7•d50. Dicha dispersión y el hecho de que ks sea varias veces superior al diámetro medio del sedimento puede atribuirse en diferente grado: a la heterogeneidad del sedimento en lechos naturales, a las formas de fondo, al transporte sólido de fondo,así como a las limitaciones del modelo logarítmico de distribución de velocidad bajo ciertas condiciones de flujo. La predicción de ks en función de variables estadísticas del campo de elevaciones del lecho se ha revelado como una alternativa con una elevada capacidad explicativa, por lo que en la medida que avancen las técnicas microtopográficas se consolidará esta vía como el método del futuro.
Resumo:
A Cu/Fe granular film, formed from a multilayer film and composed of particles of Fe imbedded in Cu, has had several of its important properties investigated. Measurements include ferromagentic resonance, magnetoresistance, Mössbauer effect, magnetic viscosity, and magnetization. The two‐phase behavior of these immiscible alloy systems, and the effect of multilayering on the shape of the magnetic precipitates, can explain some of these properties. An explanation of the ferromagnetic resonance line shape is proffered. An extraordinary macroscopic quantum tunneling effect is found to govern the magnetic relaxation at the lowest temperatures.