Application of WRF-Chem to Forecasting PM10 Concentration Over Poland

The meteorological and chemical transport model WRF-Chem was implemented to forecast PM10 concentrations over Poland. WRF-Chem version 3.5 was configured with three one-way nested domains using the GFS meteorological data and the TNO MACC II emissions. The 48 hour forecasts were run for each day of the winter and summer period of 2014 and there is only a small decrease in model performance for winter with respect to forecast lead time. The model in general captures the variability in observed PM10 concentrations for most of the stations. However, for some locations and specific episodes, the model performance is poor and the results cannot yet be used by official authorities. We argue that a higher resolution sector-based emission data will be helpful for this analysis in connection with a focus on planetary boundary layer processes in WRF-Chem and their impact on the initial distribution of emissions on both time and space.

A Parameter Estimation and Identifiability Analysis Methodology Applied to a Street Canyon Air Pollution Model

Mathematical models are increasingly used in environmental science thus increasing the importance of uncertainty and sensitivity analyses. In the present study, an iterative parameter estimation and identifiability analysis methodology is applied to an atmospheric model – the Operational Street Pollution Model (OSPMr). To assess the predictive validity of the model, the data is split into an estimation and a prediction data set using two data splitting approaches and data preparation techniques (clustering and outlier detection) are analysed. The sensitivity analysis, being part of the identifiability analysis, showed that some model parameters were significantly more sensitive than others. The application of the determined optimal parameter values was shown to succesfully equilibrate the model biases among the individual streets and species. It was as well shown that the frequentist approach applied for the uncertainty calculations underestimated the parameter uncertainties. The model parameter uncertainty was qualitatively assessed to be significant, and reduction strategies were identified.