CARS在超音速燃烧研究中的应用

报道了氮、氧和水的Q支CARS谱以及氢的S(5)和S(6)纯转动CARS的测量结果,并用来确定超音速燃烧火焰中的温度及氧的浓度;用水的Q支CARS谱得到共振与非共振谱积分面积比随浓度的变化曲线.提出并发展的同时测量氢和氧的CARS谱新方法,为同时测量火焰温度和氢、氧浓度提供了一条途径,特别对不含氮的燃烧系统更具重要意义.

Multiplex CARS measurements in supersonic H-2/air combustion

H-2 and O-2 multiplex coherent anti-stokes Raman spectroscopy (CARS) employing a single dye laser has been explored to simultaneously determine the temperature and concentrations of H-2 and O-2 in a hydrogen-fueled supersonic combustor. Systematic calibrations were performed through a well-characterized H-2/air premixed flat-flame burner. In particular, temperature measurement was accomplished using the intensity ratio of the H-2 S(5) and S(6) rotational lines, whereas extraction of the H-2 and O-2 concentrations was obtained from the H-2 S(6) and O-2 Q-branch, respectively. Details of the calibration procedure and data reduction are discussed. Quantification of the supersonic mixing and combustion characteristics applying the present technique has been demonstrated to be feasible. The associated detection limits as well as possible improvements are also identified.

氢／空气预混平面火焰CARS温度测量

介绍了一套用于燃烧研究中对温度和成分浓度测量进行校准的氢／空气预混平面火焰燃烧４系统。采用氮ＣＡＲＳ技术对氢／空气预混平面火焰温度进行了系统的测量，包括不同当量比条件下的温度分布，温度的纵向和横向空间分布。结果表明，氮ＣＡＲＳ测温与氢／空气预混平面火焰的理论计算温度之间的误差为３.４％，而在燃烧炉表面上方１ｍｍ以上的空间属于火焰的温度均匀区，温度的不均匀性约为１.８％。

同时测量氢氧CARS光谱确定火焰温度和氢氧浓度的研究

利用YAG激光器和一台染料激光器同时测量了氢/空气预混平面火焰中氢氧CARS光谱。从氢的S(5)和S(6)支纯转动线的强度比获得火焰温度，并与由氮的CARS光谱得到的温度进行了实验校验。氢和氧的浓度分别由氢的S(6)支和氧的Q支光谱求得，并利用氢/空气预混平面火焰的局部热力学平衡计算对所得浓度进行了校验。温度的校验误差为4%，而氢氧浓度的校验误差分别为14%和12%。

USED CARS测量对撞式扩散火焰的温度分布

介绍了用USED CARS技术测量对撞式甲烷/空气扩散火焰前滞止区和尾流区的温度分布剖面。在滞止区富甲烷观察到甲烷燃烧前的热解过程；尾流区温度高于滞止区温度，表明在滞止区有未完全燃烧的中间产物存在，在尾流区发现C_2及CH的光谱也证明了这一点。

同时测量氢和氧CARS谱的新方法

提出一种仅需一台染料激光器即可同时测量火焰中氢和氧的CARS谱的新方法。取带宽为120cm~(-1)，中心波长位于580.4nm的Stokes光束与532nm的泵浦光束相配合，同时测量氢扩散火焰中的氢和氧的CARS谱，用氢的S(6)和S(5)的积分强度比确定火焰中的温度并与氮的Q支CARS谱测量的温度和经过热损耗修正的热电偶测得的温度取得了相当好的一致结果。一次测出氢和氧的CARS谱，避免多次测量中参数的难以重复性，提高了以温度为参数来确定浓度的准确性。

OH在火焰中浓度分布图像及与温度关系的PLIF和CARS研究

用平面激光诱导荧光(PLIF)技术测量了平面火焰炉、狭缝火焰炉的单脉冲激光诱导OH荧光。由平面荧光图可得到氢氧基相对浓度分布和它的宽度。对扩散火焰，高温区在OH带内侧；OH带的外侧则是火焰的边界，相干反斯托克斯拉曼光谱(CARS)的测量结果对此提出了有力的佐证。湍流火焰的PLIF图则清晰地显示出火焰面的不规则性。氢氧基的PLIF图像是研究火焰结构和流场的有力工具。

环形泵浦相位匹配CARS技术的匹配方式和空间分辨率的实验研究

通过对环形泵辅相位匹配方式的解剖，发现所得到的CARS信号是由多种相让匹配方式产生的，分析了各种匹配方式产生的CARS强度的份额与空间分布。通过光路设计可得到与交叉BOXCARS相比拟的空间分辨率。计算和实验都证实了两束泵浦光与斯托克斯光在透镜表面上的张角有一最佳值，这种相位匹配方式是不存在相位失配的BOXCARS，并充分利用了环形泵浦束的能量。

The research of range-gated laser night vision system on cars - art. no. 68351V

The characteristic of several night imaging and display technologies on cars are introduced. Compared with the current night vision technologies on cars, Range-gated technology can eliminate backscattered light and increase the SNR of system. The theory of range-gated image technology is described. The plan of range-gated system on cars is designed; the divergence angle of laser can be designed to change automatically, this allows overfilling of the camera field of view to effectively attenuate the laser when necessary. Safety range of the driver is calculated according to the theory analysis. Observation distance of the designed system is about 500m which is satisfied with the need of safety driver range.

探测气体平衡及非平衡态的相干反斯托克斯喇曼散射技术

<正> 一、引言 这篇综述的目的在于介绍最近发展起来的相干反斯托克斯喇曼散射(Coherent Anti-Stokes Raman Scattering(CARS))方法在诊断平衡及非平衡态气体中的应用,包括实验及理论两部分.文内还扼要介绍了我们正在筹备的测试系统的方案。 在气体中,特别在稀薄气体非平衡流动中,探测粒子数密度分布;混合含气中各组分,各能态的分布;平动、振动、转动温度;粒子的激发和弛豫过程,都是比较困难的,而这些

Imaging properties of coherent anti-Stokes Raman scattering microscope

The coherent anti-Stokes Raman scattering (CARS) microscope with the combination of confocal and CARS techniques is a remarkable alternative for imaging chemical or biological specimens that neither fluoresce nor tolerate labelling. CARS is a nonlinear optical process, the imaging properties of CARS microscopy will be very different from the conventional confocal microscope. In this paper, the intensity distribution and the polarization property of the optical field near the focus was calculated. By using the Green function, the precise analytic solution to the wave equation of a Hertzian dipole source was obtained. We found that the intensity distributions vary considerably with the different experimental configurations and the different specimen shapes. So the conventional description of microscope (e.g. the point spread function) will fail to describe the imaging properties of the CARS microscope.