291 resultados para COULOMB DISSOCIATION


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完全电离等离子体中,当试探粒子分布函数fα是关于试探粒子速度vα的偶函数时,导出了一个新的动力学方程的碰撞算子.该碰撞算子同时包括了大角散射(库仑近碰撞)和小角散射(库仑远碰撞)的二体碰撞的贡献,因此,该碰撞算子同时适用于弱耦合(库仑对数ln∧≥10)和中等耦合(库仑对数2≤ln∧≤10)等离子体.而且经过修改的碰撞算子和Rosenbluth势有直接的联系,当试探粒子和场粒子满足条件mα<mβ(如电子-离子碰撞或Lorentz气体模型)和|vα|〉|vβ|时,经约化的电子-离子碰撞算子同最初的Fokker

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This paper reports self-organized nanostructures observed on the surface of ZnO crystal after irradiation by a focused beam of a femtosecond Ti:sapphire laser with a repetition rate of 250 kHz. For a linearly polarized femtosecond laser, the periodic nanograting structure on the ablation crater surface was promoted. The period of self-organization structures is about 180 nm. The grating orientation is adjusted by the laser polarization direction. A long range Bragg-like grating is formed by moving the sample at a speed of 10 mu m/s. For a circularly polarized laser beam, uniform spherical nanoparticles were formed as a result of Coulomb explosion during the interaction of near-infrared laser with ZnO crystal.

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Deep-subwavelength gratings with periodicities of 170, 120, and 70 nm can be observed on highly oriented pyrolytic graphite irradiated by a femtosecond (fs) laser at 800 nm. Under picosecond laser irradiation, such gratings likewise can be produced. Interestingly, the 170-nm grating is also observed on single-crystal diamond irradiated by the 800-nm fs laser. In our opinion, the optical properties of the high-excited state of material surface play a key role for the formation of the deep-subwavelength gratings. The numerical simulations of the graphite deep-subwavelength grating at normal and high-excited states confirm that in the groove the light intensity can be extraordinarily enhanced via cavity-mode excitation in the condition of transverse-magnetic wave irradiation with near-ablation-threshold fluences. This field enhancement of polarization sensitiveness in deep-subwavelength apertures acts as an important feedback mechanism for the growth and polarization dependence of the deep-subwavelength gratings. In addition, we suggest that surface plasmons are responsible for the formation of seed deep-subwavelength apertures with a particular periodicity and the initial polarization dependence. Finally, we propose that the nanoscale Coulomb explosion occurring in the groove is responsible for the ultrafast nonthermal ablation mechanism.

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The interaction of intense femtosecond laser pulses with hydrogen clusters has been experimentally studied. The hydrogen clusters were produced from expansion of high-pressure hydrogen gas (backed up to 8x10(6)Pa) into vacuum through a conical nozzle cryogenically cooled by liquid nitrogen. The average size of hydrogen clusters was estimated by Rayleigh scattering measurement and the maximum proton energy of up to 4.2keV has been obtained from the Coulomb explosion of hydrogen clusters under 2 x 10(16)W/cm(2) laser irradiation. Dependence of the maximum proton energy on cluster size and laser intensity was investigated, indicating the correlation between the laser intensity and the cluster size. The maximum proton energy is found to be directly proportional to the laser intensity, which is consistent with the theoretical prediction.

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The photoionization of H atoms irradiated by few-cycle laser pulses is studied numerically. The variations of the total ionization, the partial ionizations in opposite directions, and the corresponding asymmetry with the carrier-envelope phase in several pulse durations are obtained. We find that besides a stronger modulation on the partial ionizations, the change of pulse duration leads to a shift along carrier-envelope (CE) phase in the calculated signals. The phase shift arises from the nonlinear property of ionization and relates closely to the Coulomb attraction of the parent ion to the ionized electron. Our calculations show good agreement with the experimental observation under similar conditions.

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Self-trapping, stopping, and absorption of an ultrashort ultraintense linearly polarized laser pulse in a finite plasma slab of near-critical density is investigated by particle-in-cell simulation. As in the underdense plasma, an electron cavity is created by the pressure of the transmitted part of the light pulse and it traps the latter. Since the background plasma is at near-critical density, no wake plasma oscillation is created. The propagating self-trapped light rapidly comes to a stop inside the slab. Subsequent ion Coulomb explosion of the stopped cavity leads to explosive expulsion of its ions and formation of an extended channel having extremely low plasma density. The energetic Coulomb-exploded ions form shock layers of high density and temperature at the channel boundary. In contrast to a propagating pulse in a lower density plasma, here the energy of the trapped light is deposited onto a stationary and highly localized region of the plasma. This highly localized energy-deposition process can be relevant to the fast ignition scheme of inertial fusion.

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The triggering of wave-breaking in a three-dimensional laser plasma wake (bubble) is investigated. The Coulomb potential from a nanowire is used to disturb the wake field to initialize the wave-breaking. The electron acceleration becomes more stable and the laser power needed for self-trapping is lowered. Three-dimensional particle-in-cell simulations were performed. Electrons with a charge of about 100 pC can be accelerated stably to energy about 170 MeV with a laser energy of 460 mJ. The first step towards tailoring the electron beam properties such as the energy, energy spread, and charge is discussed. (C) 2007 American Institute of Physics.

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利用一简单的经典静电模型研究了甲烷团簇纯库仑爆炸情况下产生的离子平均动能。研究表明,甲烷团簇爆炸后离子获得的平均动能和离子的初始平均静电势能的比值,与团簇的尺寸大小无关。这意味着在甲烷团簇纯库仑爆炸近似下,不必使用分子动力学模拟,离子获得的动能可以通过这一比值以及离子的初始静电势能进行估算。给出了不同碳离子价态下的离子平均动能和其初始平均静电势能的比值。

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Two basic types of depolarization mechanisms, carrier-carrier (CC) and carrier-phonon (CP) scattering, are investigated in optically excited bulk semiconductors (3D), in which the existence of the transverse relaxation time is proven based on the vector property of the interband transition matrix elements. The dephasing rates for both CC and CP scattering are determined to be equal to one half of the total scattering-rate-integrals weighted by the factors (1 - cos chi), where chi are the scattering angles. Analytical expressions of the polarization dephasing due to CC scattering are established by using an uncertainty broadening approach, and analytical ones due to both the polar optical-phonon and non-polar deformation potential scattering (including inter-valley scattering) are also presented by using the sharp spectral functions in the dephasing rate calculations. These formulas, which reveal the trivial role of the Coulomb screening effect in the depolarization processes, are used to explain the experimental results at hand and provide a clear physical picture that is difficult to extract from numerical treatments.

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Based on the Coulomb friction model, the frictional motion model of workpiece relating to the polishing pad was presented in annular polishing. By the dynamic analysis software, the model was simulated and analysed. The conclusions from the results were that the workpiece did not rotate steadily. When the angular velocity of ring and the direction were the same as that of the polishing pad, the angular velocity of workpiece hoicked at the beginning and at the later stage were the same as that of the polishing pad before contacting with the ring. The angular velocity of workpiece vibrated at the moment of contacting with the ring. After that the angular velocity of workpiece increased gradually and fluctuated at a given value, while the angular velocity of ring decreased gradually and also fluctuated at a given value. Since the contact between the workpiece and the ring was linear, their linear velocities and directions should be the same. But the angular velocity of workpiece was larger than that of the polishing pad on the condition that the radius of the workpiece was less than that of the ring. This did not agree with the pure translation principle and the workpiece surface could not be flat, either. Consequently, it needed to be controlled with the angular velocity of ring and the radii of the ring and the workpiece, besides friction to make the angular velocity of workpiece equal to that of the polishing pad for obtaining fine surface flatness of the workpiece. Copyright © 2007 Inderscience Enterprises Ltd.}

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本文基于库仑摩擦模型,模拟了不同形状的工件在环形抛光的运动。从结果可知,(1)如果工作环处于自由转动状态,工件的角速度在环形抛光中比抛光盘的角速度大;(2)可通过控制工作环的角速度使工件和抛光盘的角速度同步。工作环的角速度依赖于工作环和工件的半径、抛光盘-工件和抛光盘-工作环的摩擦系数,以及抛光盘的角速度;(3)有尖角的工件与工作环的接触处于不连续状态,导致二者的接触状态发生变化和工件角速度的波动。

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A series of ZnO thin films were deposited on ZnO buffer layers by DC reactive magnetron sputtering. The buffer layer thickness determination of microstructure and optical properties of ZnO films was investigated by X-ray diffraction (XRD), photoluminescence (PL), optical transmittance and absorption measurements. XRD results revealed that the stress of ZnO thin films varied with the buffer layer thickness. With the increase of buffer layer thickness, the band gap edge shifted toward longer wavelength. The near-band-edge (NBE) emission intensity of ZnO films deposited on ZnO buffer layer also varied with the increase of thickness due to the spatial confinement increasing the Coulomb interaction between electrons and holes. The PL measurement showed that the optimum thickness of the ZnO buffer layer was around 12 nm. (c) 2005 Elsevier B.V. All rights reserved.

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一,螺旋藻藻胆体光谱特性及其光能传递的研究 1,完整藻胆体与解离藻胆体吸收光谱的比较研究 对螺旋藻完整藻胆体和解离藻胆体的吸收光谱中进行了比较研究。随着PBS逐渐解离,其吸收光谱表现出如下变化特点:在紫外区,吸收峰始终位于355nm,尖形峰逐渐变成钝形峰;在红区,完整藻胆体和解离藻胆体都有很强的光吸收,吸收峰呈平顶状,其半带宽逐渐变小,紫外区与红区相对吸收强度比值逐渐变小,四组导数吸收光谱中的小峰数目越来越少。室温荧光发射光谱表明,PBS在低于0.9mol/L的磷酸缓冲液中变得不稳定,并开始逐渐解离,解离的PBS与完整的PBS相比,其荧光发射峰逐渐蓝移。 2,藻胆体在解离过程中荧光发射和光能传递的研究 完整藻胆体的室温荧光发射光谱中只有一个峰,在678nm。说明在完整藻胆体中,光能传递效率高。在77K荧光发射光谱中,完整藻胆体只有一个峰,位于682nm,这是L_(cm)(TE_1)的荧光峰;严重解离的藻胆体的主峰在656nm,是PC的荧光;在679nm有一个小峰,是APC-B的荧光(TE_2)。据此,我们提出螺旋藻藻胆体的光能传递链为:(此处表从略,见全文) 二,螺旋藻藻胆体核心及其与藻蓝蛋白的重组 PC+core混合物,浓缩重组48h后,其室温荧光发射峰位于663nm,与PC的室温荧光发射峰643nm和PC+core混合物(未重组)的室温荧光发射峰648nm相比,说明部分APC与部分PC发生了重组,使部分PC吸收的光能传递给了APC,使荧光发射峰红移;与藻胆体核心室温荧光发射峰664nm相比,则非常接近,说明重组效果较好。PC+core混合物(未重组),其77K荧光发射光谱中有两个峰:654nm,679nm,分别是PC,APC-B的荧光峰,F679/F654的比值为32.0%。我们以F679/F654比值的变化来判断PC与core是否发生了重组。PC+core混合物,经48h浓缩重组后,77K荧光发射光谱中有F657,F679两个峰,F679/F654的比值则为45.9%,比未重组的混合物32.0%升高了,说明部分PC与core发生了重组,部分PC吸收的光能传递给了APC和APC-B,使F679加强,F654减弱。 三,螺旋藻藻胆体一类囊体膜光谱特性与光能传递的研究 藻胆体一类囊体膜的吸收光谱,室温荧光发射光谱和77K荧光发射光谱表明:藻胆蛋白能将捕获的光能传递给叶绿素a,叶绿素a捕获的光能不能逆传给藻胆蛋白。 四,藻胆体一类囊体膜的重组 藻胆体一类囊体膜的吸收光谱说明,一部分被洗下来的PBS能重新结合到类囊体膜上,但并没有达到100%的重组。 五,整体螺旋藻光谱特性及其光能传递的研究 整体螺旋藻光谱特性与PBS-类囊体膜的光谱特性极为相似,表现出同样的规律:PBS的吸收面积与叶绿素a相比,叶绿素a的吸收是主要的。 从PBS-类囊体膜和整体螺旋藻的吸收光谱,室温荧光发射光谱,77K荧光发射光谱的研究中可知,二者表现出极为相似的规律:PBS藻胆蛋白捕获的光能能传递给叶绿素a,叶绿素a捕获的光能不能逆传给PBS藻胆蛋白。主要的捕光物质是叶绿素a。 另外,我们还对Spirulina platensis 6 and Spirulina maxima的藻胆体在解离过程中的荧光发射和光能传递进行了研究,表现规律与Spirulina platensis相同。

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A novel potent trypsin inhibitor was purified and characterized from frog Bombina maxima skin. A full-length cDNA encoding the protein was obtained from a cDNA library constructed from the skin. Sequence analysis established that the protein actually comprises three conserved albumin domains. B. maxima serum albumin was subsequently purified, and its coding cDNA was further obtained by PCR-based cloning from the frog liver. Only two amino acid variations were found in the albumin sequences from the skin and the serum. However, the skin protein is distinct from the serum protein by binding of a haem b (0.95 mol/mol protein). Different from bovine serum albumin, B. maxima albumin potently inhibited trypsin. It bound tightly with trypsin in a 1: 1 molar ratio. The equilibrium dissociation constants (K-D) obtained for the skin and the serum proteins were 1.92 x 10(-9) M and 1.55 x 10(-9) M, respectively. B. maxima albumin formed a noncovalent complex with trypsin through an exposed loop formed by a disulfide bond (Cys(53)-Cys(62)), which comprises the scissile bond Arg(58)(P-1)-His(59)(P-1'). No inhibitory effects on thrombin, chymotrypsin, elastase, and subtilisin were observed under the assay conditions. Immunohistochemical study showed that B. maxima albumin is widely distributed around the membranes of epithelial layer cells and within the stratum spongiosum of dermis in the skin, suggesting that it plays important roles in skin physiological functions, such as water economy, metabolite exchange, and osmoregulation.

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This research is focused on the contribution of area 7 to the short-term visual spatial memory. Three rhesus monkeys (Macaca mulatta) were trained in the direct delayed response task in which 5 delay intervals were used in each session. When each monkey reached the criterion of 90% correct responses in 5 successive sessions, two monkeys underwent a surgery while the other one received a sham operation as a control. In the first stage of the surgery, bilateral areas 7a, 7b and 7ip of the parietal cortex of two monkeys were precisely lesioned. After 7 days of recuperation, the monkeys were required to do the same task. The average percentage of correct responses in the lesioned animals decreased from 94.7% to 89.3% and 93.3% to 82.0% respectively (no significance, P > 0.05, n = 2). In addition, the monkeys' complex movements were mildly impaired. The lesioned monkeys were found to have difficulty picking up food from the wells. In the second stage, bilateral area 7m was lesioned. In the 5 postoperative sessions, the average percentage of correct responses in one monkey, with a relatively precise 7m lesion, decreased from 94.7% to 92.2% (no significance, P > 0.05), while the other monkey, with widely spread necrosis of lateral parietal cortex, showed an. obvious decline in performance, but still over the chance level. After 240 trials this monkey reattained the normal criterion. The results of this research suggest that the lesions of area 7 of the parietal cortex did not significantly affect the short-term visual spatial memory, which has been shown to be sensitive to lesions of the prefrontal cortex; they also support the notion of dissociation of spatial functions in the prefrontal and parietal cortices.