Experimental Study of Surface Deformation and Flow Pattern on Buoyant-Thermocapillary Convection

Free surface deformation is one of the most important physical phenomena in fluids with free surface. In the present paper, convection and surface deformation caused by thermocapillary effect in a rectangular cavity were investigated. In ground experiments, the convection was also affected by gravity. The cavity has a horizontal cross section of 52mm×42mm and the thikkness of the liquid layer is 4mm. Temperature difference between two sides of the liquid layer was increased gradually, and the flow in liquid layer will develop from steady to unstable convection. An optical diagnostic system consisting of a revised Michelson interferometer with image processor was developed to study fluid surface deformation in convection, and the displacements of free surface oscillation were determined. PIV technique was adopted to observe the evolution of flow pattern, and the velocity fields were obtained quantitatively. The present experiments demonstrate that surface deformation is quite distinct in buoyant-thermocapillary convection. in order to understand the mechanism of buoyant-thermocapillary convection, not only the hydrothermal wave instability but also the surface wave instability should be discussed.

Thermocapillary Convection in Floating Zones

This paper provides an overview of ongoing studies in the area of thermocapillary convection driven by a surface tension gradient parallel to the free surface in a floating zone. Here, research interests are focused around the onset of oscillatory thermocapillary convection, also known as the transition from quasisteady convection to oscillatory convection. The onset of oscillation depends on a set of critical parameters, and the margin relationship can be represented by a complex function of the critical parameters. The experimental results indicate that the velocity deviation of an oscillatory flow has the same order of magnitude as that of an average flow, and the deviations of other quantities, such as temperature and free surface radii fluctuations, are much smaller when compared with their normal counterparts. Therefore, the onset of oscillation should be a result of the dynamic process in a fluid, and the problem is a strongly nonlinear one. In the past few decades, several theoretical models have been introduced to tackle the problem using analytical methods, linear instability analysis methods, energy instability methods, and unsteady 3D numerical methods. The last of the above mentioned methods is known to be the most suitable for a thorough analysis of strong nonlinear processes, which generally leads to a better comparison with the experimental results. The transition from oscillatory thermocapillary convection to turbulence falls under the studies of chaotic behavior in a new system, which opens a fascinating new frontier in nonlinear science, a hot research area drawing many recent works. This paper reviews theoretical models and analysis, and also experimental research, on thermocapillary connection in floating zones. It cites 93 references.

Hydrothermal Instability Of Thermocapillary Convection In Large-Prandtl-Number Liquid Bridges Under Microgravity

Linear stability analysis was performed to study the mechanism of transition of thermocapillary convection in liquid bridges with liquid volume ratios ranging from 0.4 to 1.2, aspect ratio of 0.75 and Prandtl number of 100. 2-D governing equations were solved to obtain the steady axi-symmetric basic flow and temperature distributions. 3-D perturbation equations were discretized at the collocation grid points using the Chebyshev-collocation method. Eigenvalues and eigenfunctions were obtained by using the Q-R. method. The predicted critical Marangoni numbers and critical frequencies were compared with data from space experiments. The disturbance of the temperature distribution on the free surface causes the onset of oscillatory convection. It is shown that the origin of instability is related to the hydrothermal origin for convections in large-Prandtl-number liquid bridges. (C) 2007 COSPAR. Published by Elsevier Ltd. All rights reserved.

Coupling Of Evaporation And Thermocapillary Convection In A Liquid Layer With Mass And Heat Exchanging Interface

We propose and analyse a new model of thermocapillary convection with evaporation in a cavity subjected to horizontal temperature gradient, rather than the previously studied model without evaporation. The pure liquid layer with a top free surface in contact with its own vapour is considered in microgravity condition. The computing programme developed for simulating this model integrates the two-dimensional, time-dependent Navier-Stokes equations and energy equation by a second-order accurate projection method. We focus on the coupling of evaporation and thermocapillary convection by investigating the influence of evaporation Biot number and Marangoni number on the interfacial mass and heat transfer. Three different regimes of the coupling mechanisms are found and explained from our numerical results.

Transition of oscillatory floating half zone convection from Earth's gravity to microgravity

Oscillatory features of floating half zone convection were experimentally studied by using the drop shaft facility of Japan Microgravity Center which supported microgravity period of 10 s. Coordinated measurements including free surface deformation and oscillation, temperature and flow pattern in both 1-g and micro-g environment were obtained. The oscillatory frequency and amplitude in micro-g condition were lower and larger than the ones in l-g condition, respectively. The results gave, at first time, the oscillatory features such as free surface wave in micro-g, coordinated measurements of more than two physical quantities in the micro-g, and transition of thermocapillary oscillatory convection from I-g to micro-g.

Numerical investigation on a simulation model of floating zone convection

A simulation model with adiabatic condition at the upper rod and constant temperature at the lower rod is studied numerically in this paper. The temperature distribution in a simulation model is closer to the one in the half part of a floating full zone in comparison with the one in a usual floating half zone model with constant temperature at both rods, because the temperature distribution of a floating full zone is symmetric for the middle plane in a microgravity environment. The results of the simulation model show that the temperature profiles and the how patterns are different from those of the usual floating half zone model. Another type of half zone model, with a special non-uniform temperature distribution at the upper rod and constant temperature at the lower rod, has been suggested by recent experiments. The temperature boundary condition of the upper rod has a maximum value in the center and a lower value near the free surface. This modified simulation model is also simulated numerically in the present paper. Copyright (C)1996 Elsevier Science Ltd.

Numerical simulation of g-jitter effects on half floating zone convection under microgravity environment

The g-jitter effects on the thermocapillary convection in liquid bridge of floating half zone were studied by numerical simulation for unsteady and axi-symmetric model in the cylindrical coordinate system. The g-jitter field was given by a steady microgravity field in addition to an oscillatory low-gravity field, and the effects on the flow field, temperature distribution and free surface deformation were analyzed numerically.

How to determine critical Marangoni number in half floating zone convection

In the present paper, the coordinated measurements of the temperature profile inside the liquid bridge and the boundary variation of Free surface, in addition to other quantities, were obtained in the same time for the half floating zone convection. The results show that the onset of free surface oscillation is earlier than the one of temperature oscillation during the increasing of applied temperature difference, and the critical Marangoni numbers, defined usually by temperature measurement, are larger than the one defined by free surface measurement, and the difference depends on the volume of liquid bridge. These results induce the question, ''How to determine experimentally the critical Marangoni number?'' Copyright (C) 1996 Elsevier Science Ltd.

Hardware development and ground-based studies for drop shaft experiment on oscillatory convection in half floating-zone

Coordinated measurement of temperature, velocity and free surface oscillation were obtained by using the drop shaft facility for microgravity experiments of half floating zone convection. The ground-based studies gave transition from steady to oscillatory convection for multi-quantities measurement.

G-jitter effects on half floating-zone convection in intermediate-frequency range

The g-jitter influence on thermocapillary convection and critical Marangoni number in a liquid bridge of half-floating rone was discussed in the low frequency range of 0.4 to 1.5 Hz in a previous paper. This paper extended the experiments to the intermediate frequency range of 2 to 18 Hz, which htrs often been recorded as vibration environment of spacecrafts. The experiment was completed on the deck of a vibration machine, which gave a periodical applied acceleration to simulate the effects of g-jitter. The experimental results in the intermediate frequency range are different from that in the low frequency range. The velocity field and the shape of the free surface have periodical fluctuations in response to g-jitter. The amplitude of the periodical varying part of the temperature response decreases obviously with increasing frequency of g-jitter and vanishes almost when the frequency of g-jitter is high enough. The critical Marangoni number is defined to describe the transition from a periodical convection in response to g-jitter to an oscillatory convection due to internal instability, and will increase with increasing g-jitter frequency. According to the spectral analysis, it can be found that the oscillatory part of temperature is a superposition of two harmonic waves if the Marangoni number is larger than a critical value.

Influence of buoyancy on floating-zone convection of small bond number

Gravity may influence the velocity and temperature distributions, bouyancy may induce Rayleigh instability and the instability may be excited due to the change of free surface shape associating with gravity in the thermocapillary convection. These effects have been studied in the present paper. The results show that gravity may have an important effect in thermocapillary oscillatory convection even for the cases of small Bond number experiments either on the ground or in space.

Experimental study on oscillatory thermocapillary convection

The transition processes from steady flow into oscillatory flow in a liquid bridge of the half floating zone are studied experimentally. Two methods of noncontacted diagnoses are developed to measure the distribution of critical Marangoni numbers described by the onset of the oscillation st the free surface of the liquid bridge.The experimental results obtained for both cases of the upper rod heated and the lower rod heated agree with the prediction by Rayleigh's instability theory.The sensitive relations between the relatively fat or slender liquid bridge and the onset of oscillatory convection are also discussed to reveal the insight of the pressure distribution near the free surface. The experiments have been performed in a small liquid bridge, where the Bond number is much smaller than 1, and the results can be used to simulate the experiment in the microgravity environment.

Effects of Thermocapillary Convection on the Growth Process in Industrial 8-inch Silicon Czochralski Growth

Czochralski (CZ) crystal growth process is a widely used technique in manufacturing of silicon crystals and other semiconductor materials. The ultimate goal of the IC industry is to have the highest quality substrates, which are free of point defect, impurities and micro defect clusters. The scale up of silicon wafer size from 200 mm to 300 mm requires large crucible size and more heat power. Transport phenomena in crystal growth processes are quite complex due to melt and gas flows that may be oscillatory and/or turbulent, coupled convection and radiation, impurities and dopant distributions, unsteady kinetics of the growth process, melt crystal interface dynamics, free surface and meniscus, stoichiometry in the case of compound materials. A global model has been developed to simulate the temperature distribution and melt flow in an 8-inch system. The present program features the fluid convection, magnetohydrodynamics, and radiation models. A multi-zone method is used to divide the Cz system into different zones, e.g., the melt, the crystal and the hot zone. For calculation of temperature distribution, the whole system inside the stainless chamber is considered. For the convective flow, only the melt is considered. The widely used zonal method divides the surface of the radiation enclosure into a number of zones, which has a uniform distribution of temperature, radiative properties and composition. The integro-differential equations for the radiative heat transfer are solved using the matrix inversion technique. The zonal method for radiative heat transfer is used in the growth chamber, which is confined by crystal surface, melt surface, heat shield, and pull chamber. Free surface and crystal/melt interface are tracked using adaptive grid generation. The competition between the thermocapillary convection induced by non-uniform temperature distributions on the free surface and the forced convection by the rotation of the crystal determines the interface shape, dopant distribution, and striation pattern. The temperature gradients on the free surface are influenced by the effects of the thermocapillary force on the free surface and the rotation of the crystal and the crucible.

Floating zone convection

The microgravity research, as a branch of the advanced sciences and a spe- cialized field of high technology, has been made in China since the late 1980's. The research group investigating microgravity fluid physics consisted of our col- leagues and the authors in the Institute of Mechanics of the Chinese Academy of Sciences (CAS), and we pay special attention to the floating zone convection as our first research priority. Now, the research group has expanded and is a part of the National Microgravity Laboratory of the CAS, and the research fields have been extended to include more subjects related to microgravity science. Howev- er, the floating zone convection is still an important topic that greatly holds our research interests.

Effect of interfacial heat transfer on the onset of oscillatory convection in liquid bridge

In present study, effect of interfacial heat transfer with ambient gas on the onset of oscillatory convection in a liquid bridge of large Prandtl number on the ground is systematically investigated by the method of linear stability analyses. With both the constant and linear ambient air temperature distributions, the numerical results show that the interfacial heat transfer modifies the free-surface temperature distribution directly and then induces a steeper temperature gradient on the middle part of the free surface, which may destabilize the convection. On the other hand, the interfacial heat transfer restrains the temperature disturbances on the free surface, which may stabilize the convection. The two coupling effects result in a complex dependence of the stability property on the Biot number. Effects of melt free-surface deformation on the critical conditions of the oscillatory convection were also investigated. Moreover, to better understand the mechanism of the instabilities, rates of kinetic energy change and "thermal" energy change of the critical disturbances were investigated (C) 2009 Elsevier Ltd. All rights reserved.