6 resultados para radionucléides

em Aquatic Commons


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Radioactivity measured in samples from the NEA-Dumping-Site not only emanated from dumped barrels. Just as everywhere on the world also fallout from former nuclear weapon tests can be found there. Radionuclides which can emanate from different sources do not tell anything about their origin. To assess the fractions from various sources activity ratios from radionuclides can be used. There are different activity ratios for fallout and for waste from peaceful nuclear power engeneering. The comparison of the ratios of the plutonium isotopes Pu-238 and the sum of Pu-239 and Pu-240 (Pu-238/Pu-239,240) in benthic samples from the dumping site and from reference sites without waste dumping gives a clear hint. In the sampling period from 1980 to 2000 for samples from the dumping site this ratio increases significantly from 1986 on. Radioactivity emanating from the dumped barrels is regarded as causing this.

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A subject of a change of authorised limits in 1994 for the discharge of liquid radioactive waste by the reprocessing plant Sellafield (UK) was an increase of these limits for certain radionuclides (3H, 14C, 60Co, 99Tc and 129I). It is investigated now how the radioactivity in marine biota from the North Sea and subsequently the public radiation exposure by ingestion has developed in the years since 1994. This is based on a compartment model for the Northeast Atlantic. Discharges of the reprocessing plants Dounreay (UK) and La Hague (F) are included in the assessment. It is deduced that about 60 % of 137Cs in the North Sea originate presently in the remobilisation of old Sellafield discharges from the Irish Sea sediment. A comparison with measured biota data shows that the model is conservative in the most cases. The public radiation exposure from ingestion of fish, crustaceans and molluscs from the central North Sea as the sum over 12 considered radionuclides has decreased from 1992 to 1998 from 0,13 to 0,08 μSv·y–1. For the southward and northward joined regions it was a little bit smaller with a similar decreasing trend.

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The identification of artificial radionuclides in fish involves some diffculties, because the quantities of these nuclides are very low (10-16 to 10-10 g/kg). The procedures have to be done very carefully. The sample preparation, the radiochemical analyses and the final preparation of the samples for the detection of the radioactivity of strontium-90, plutonium-238, -239, -240 and americium-241 are briefly described. The levels of artificial radioactivity in some species of fish from the North Sea are shown. The additional exposure to radiation by artificial radionuc1ides by ingestion of fish amounts only to about 0,02 % of the mean exposure to natural radiation. Nevertheless further monitoring of radioactivity should be continued in order to ensure that changes can be detected in time.

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This is the Impact Assessment of ionising Radiation on Wildlife document produced by the Environment Agency in 2001. This report describes the behaviour and transport of radionuclides in the environment, considers the impact of ionising radiation on wildlife, and makes recommendations on an approach for the Impact assessment of ionising radiation on wildlife for England and Wales. The assessment approach focuses on three ecosystems representative of those considered potentially most at risk from the impact of authorised radioactive discharges, namely a coastal grassland (terrestrial ecosystem); estuarine and freshwater ecosystems. The likely scale of the impact on wildlife is also assessed in light of a preliminary analysis based on this assessment approach. The report demonstrates the behaviour and transfer of radionuclides in a number of different ecosystem types. Particular emphasis is placed on exposure pathways in those ecosystems most likely to be impacted by the authorised discharges of radioactivity within England and Wales. The use of biomarker techniques is reviewed in the report, and their application to the study of exposure to multiple contaminants is discussed.

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Low level aqueous radioactive wastes from the nuclear complex at Trombay are discharged into the Bombay harbour. Of the 6 principal radionuclides comprising the discharge, cesium-137 is most predominantly taken up by silt from the sea water. Isoactivity contours show that activity levels just off the point of discharge, and further south to Pir Pau, were between 50 and 100 pCi/g. Activity in the main channel of the harbour remained below 10 pCi/g, while further north (below the Thane Creek bridge) it was around 20 pCi/g. Activity in the top 6 cm of a core off Trombay naval jetty was <5 pCi/g, reaching a maximum of 178 pCi/g at 14cm below the surface. Thereafter, it tapered off to 5 pCi/g down to a metre.

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Three spatial structure groups of radionuclides in U and Th series, 210Pb-excess and 137Cs, and 40K were found based on analyzing temporal and spatial datum of their content by factor analysis with oblique rotation in Nhatrang bay. U and Th spatial structure with their contours decreased toward the offshore, ran longshore and divided seawater of bay into two parts with strong gradient on both sides. Inside part located from center of Nhatrang bay toward the seashore with three main deposit centers of their contents higher than 23 Bq/kg.dry for 238U and 40 Bq/kg.dry for 232Th, indicated unstability of shoreline. Almost sediments coming from river extended toward the offshore, were stopped and transported toward southeastern. The outside part was less than above mentioned content. The boundary line between two parts superposed with the constantly limit line of turbid plume in the rainy season. Direct influence of the continental runoff was limited by the 9 Bq/kg.dry contour of 238U, 19 Bq/kg.dry contour of 232Th. Longshore current was a predominant process whereas lateral transport as sifting and winnowing process of finer grains in sediments of Nhatrang bay. Areas that had very low content of 137Cs and 210 Pb-excess adjoining shoreline showed areas being eroded. Accumulation of 137Cs and 210 Pbexcess nearby river mouth characterized for fine compositions of sediments controlled by seasonal plumes and sites further toward the south indicated finer materials transported from river and accumulated in lack of hydrodynamic process. Near shore accumulation of 40K revealed the sediments there originated from bed erosion.