Suppression of spatiotemporal chaos in the oscillatory CO oxidation on Pt(110) by focused laser light
Data(s) |
30/04/2008
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Resumo |
Chemical turbulence in the oscillatory catalytic CO oxidation on Pt(110) is suppressed by means of focused laser light. The laser locally heats the platinum surface which leads to a local increase of the oscillation frequency, and to the formation of a pacemaker which emits target waves. These waves slowly entrain the medium and suppress the spatiotemporal chaos present in the absence of laser light. Our experimental results are confirmed by a detailed numerical analysis of one- and two-dimensional media using the Krischer-Eiswirth-Ertl model for CO oxidation on Pt110. Different control regimes are identified and the dispersion relation of the system is determined using the pacemaker as an externally tunable wave source. |
Formato |
application/pdf |
Identificador |
Punckt, Christian; Stich, Michael; Beta, Carsten and Rotermund, Harm Hinrich (2008). Suppression of spatiotemporal chaos in the oscillatory CO oxidation on Pt(110) by focused laser light. Physical Review E, 77 (4), |
Relação |
http://eprints.aston.ac.uk/20339/ |
Tipo |
Article PeerReviewed |