Morphological changes in convection-diffusion-limited deposition
Contribuinte(s) |
Universitat de Barcelona |
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Data(s) |
04/05/2010
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Resumo |
The effect of hydrodynamic flow upon diffusion-limited deposition on a line is investigated using a Monte Carlo model. The growth process is governed by the convection and diffusion field. The convective diffusion field is simulated by the biased-random walker resulting from a superimposed drift that represents the convective flow. The development of distinct morphologies is found with varying direction and strength of drift. By introducing a horizontal drift parallel to the deposition plate, the diffusion-limited deposit changes into a single needle inclined to the plate. The width of the needle decreases with increasing strength of drift. The angle between the needle and the plate is about 45° at high flow rate. In the presence of an inclined drift to the plate, the convection-diffusion-limited deposit leads to the formation of a characteristic columnar morphology. In the limiting case where the convection dominates, the deposition process is equivalent to ballistic deposition onto an inclined surface. |
Identificador | |
Idioma(s) |
eng |
Publicador |
The American Physical Society |
Direitos |
(c) The American Physical Society, 1991 info:eu-repo/semantics/openAccess |
Palavras-Chave | #Electroquímica #Física estadística #Processos estocàstics #Electrochemistry #Statistical physics #Stochastic processes |
Tipo |
info:eu-repo/semantics/article |