Evidence for a glassy state in strongly driven carbon


Autoria(s): Brown, C. R. D.; Gericke, D. O.; Cammarata, M.; Cho, B. I.; Doeppner, T.; Engelhorn, K.; Foerster, E.; Fortmann, C.; Fritz, D.; Galtier, E.; Glenzer, S. H.; Harmand, M.; Heimann, P.; Kugland, N. L.; Lamb, D. Q.; Lee, H. J.; Lee, R. W.; Lemke, H.; Makita, M.; Moinard, A.; Murphy, C. D.; Nagler, B.; Neumayer, P.; Plagemann, K. -U.; Redmer, R.; Riley, D.; Rosmej, F. B.; Sperling, P.; Toleikis, S.; Vinko, S. M.; Vorberger, J.; White, Steven; White, T. G.; Wunsch, K.; Zastrau, U.; Zhu, D.; Tschentscher, T.; Gregori, G.
Data(s)

09/06/2014

Resumo

<p>Here, we report results of an experiment creating a transient, highly correlated carbon state using a combination of optical and x-ray lasers. Scattered x-rays reveal a highly ordered state with an electrostatic energy significantly exceeding the thermal energy of the ions. Strong Coulomb forces are predicted to induce nucleation into a crystalline ion structure within a few picoseconds. However, we observe no evidence of such phase transition after several tens of picoseconds but strong indications for an over-correlated fluid state. The experiment suggests a much slower nucleation and points to an intermediate glassy state where the ions are frozen close to their original positions in the fluid.</p>

Identificador

http://pure.qub.ac.uk/portal/en/publications/evidence-for-a-glassy-state-in-strongly-driven-carbon(7ac75fa2-0f37-4733-9e25-be8aa7cbac45).html

http://dx.doi.org/10.1038/srep05214

Idioma(s)

eng

Direitos

info:eu-repo/semantics/restrictedAccess

Fonte

Brown , C R D , Gericke , D O , Cammarata , M , Cho , B I , Doeppner , T , Engelhorn , K , Foerster , E , Fortmann , C , Fritz , D , Galtier , E , Glenzer , S H , Harmand , M , Heimann , P , Kugland , N L , Lamb , D Q , Lee , H J , Lee , R W , Lemke , H , Makita , M , Moinard , A , Murphy , C D , Nagler , B , Neumayer , P , Plagemann , K -U , Redmer , R , Riley , D , Rosmej , F B , Sperling , P , Toleikis , S , Vinko , S M , Vorberger , J , White , S , White , T G , Wunsch , K , Zastrau , U , Zhu , D , Tschentscher , T & Gregori , G 2014 , ' Evidence for a glassy state in strongly driven carbon ' Scientific Reports , vol 4 , 5214 . DOI: 10.1038/srep05214

Palavras-Chave #FREE-ELECTRON LASER #PLASMAS #SCATTERING #INTERIORS #GRAPHITE #SYSTEM #MATTER #MODEL
Tipo

article