Nonlinear hydrodynamics of a hard-sphere fluid near the glass transition


Autoria(s): Lust, Lisa M; Valls, Oriol T; Dasgupta, Chandan
Data(s)

01/09/1993

Resumo

We conduct a numerical study of the dynamic behavior of a dense hard-sphere fluid by deriving and integrating a set of Langevin equations. The statics of the system is described by a free-energy functional of the Ramakrishnan-Yussouff form. We find that the system exhibits glassy behavior as evidenced through a stretched exponential decay and a two-stage relaxation of the density correlation function. The characteristic times grow with increasing density according to the Vogel-Fulcher law. The wave-number dependence of the kinetics is extensively explored. The connection of our results with experiment, mode-coupling theory, and molecular-dynamics results is discussed.

Formato

application/pdf

Identificador

http://eprints.iisc.ernet.in/35633/1/Hard.pdf

Lust, Lisa M and Valls, Oriol T and Dasgupta, Chandan (1993) Nonlinear hydrodynamics of a hard-sphere fluid near the glass transition. In: Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics, 48 (3). 1787-1798 .

Publicador

The American Physical Society

Relação

http://pre.aps.org/abstract/PRE/v48/i3/p1787_1

http://eprints.iisc.ernet.in/35633/

Palavras-Chave #Physics
Tipo

Journal Article

PeerReviewed