Second harmonic generation in<em> h</em>-BN and MoS<sub>2</sub> monolayers: Role of electron-hole interaction


Autoria(s): Grüning, M.; Attaccalite, C.
Data(s)

15/02/2014

Resumo

We study second-harmonic generation in h-BN and MoS$_2$ monolayers using a novel \emph{ab initio} approach based on Many-body theory. We show that electron-hole interaction doubles the signal intensity at the excitonic resonances with respect to the contribution from independent electronic transitions. This implies that electron-hole interaction is essential to describe second-harmonic generation in those materials. We argue that this finding is general for nonlinear optical properties in nanostructures and that the present methodology is the key to disclose these effects.

Formato

application/pdf

Identificador

http://pure.qub.ac.uk/portal/en/publications/second-harmonic-generation-in-hbn-and-mos2-monolayers-role-of-electronhole-interaction(fb2c6cf6-64d1-4da8-acdd-d1726cf01c05).html

http://dx.doi.org/10.1103/PhysRevB.89.081102

http://pure.qub.ac.uk/ws/files/11273717/second.pdf

Idioma(s)

eng

Direitos

info:eu-repo/semantics/openAccess

Fonte

Grüning , M & Attaccalite , C 2014 , ' Second harmonic generation in h -BN and MoS 2 monolayers: Role of electron-hole interaction ' Physical Review B (Condensed Matter) , vol 89 , no. 9 , 081102 . DOI: 10.1103/PhysRevB.89.081102

Tipo

article