Characterisation of the impact of open biomass burning on urban air quality in Brisbane, Australia


Autoria(s): He, Congrong; Miljevic, Branka; Crilley, Leigh R.; Surawski, Nicholas C.; Bartsch, Jennifer; Salimi, Farhad; Uhde, Erik; Schnelle-Kreis, Jürgen; Orasche, Jürgen; Ristovski, Zoran; Ayoko, Godwin A.; Zimmermann, Ralf; Morawska, Lidia
Data(s)

2016

Resumo

Open biomass burning from wildfires and the prescribed burning of forests and farmland is a frequent occurrence in South-East Queensland (SEQ), Australia. This work reports on data collected from 10-30 September 2011, which covers the days before (10-14 September), during (15-20 September) and after (21-30 September) a period of biomass burning in SEQ. The aim of this project was to comprehensively quantify the impact of the biomass burning on air quality in Brisbane, the capital city of Queensland. A multi-parameter field measurement campaign was conducted and ambient air quality data from 13 monitoring stations across SEQ were analysed. During the burning period, the average concentrations of all measured pollutants increased (from 20% to 430%) compared to the non-burning period (both before and after burning), except for total xylenes. The average concentration of O3, NO2, SO2, benzene, formaldehyde, PM10, PM2.5 and visibility-reducing particles reached their highest levels for the year, which were up to 10 times higher than annual average levels, while PM10, PM2.5 and SO2 concentrations exceeded the WHO 24-hour guidelines and O3 concentration exceeded the WHO maximum 8-hour average threshold during the burning period. Overall spatial variations showed that all measured pollutants, with the exception of O3, were closer to spatial homogeneity during the burning compared to the non-burning period. In addition to the above, elevated concentrations of three biomass burning organic tracers (levoglucosan, mannosan and galactosan), together with the amount of non-refractory organic particles (PM1) and the average value of f60 (attributed to levoglucosan), reinforce that elevated pollutant concentration levels were due to emissions from open biomass burning events, 70% of which were prescribed burning events. This study, which is the first and most comprehensive of its kind in Australia, provides quantitative evidence of the significant impact of open biomass burning events, especially prescribed burning, on urban air quality. The current results provide a solid platform for more detailed health and modelling investigations in the future.

Formato

application/pdf

Identificador

http://eprints.qut.edu.au/95275/

Publicador

Elsevier

Relação

http://eprints.qut.edu.au/95275/3/95275.pdf

DOI:10.1016/j.envint.2016.02.030

He, Congrong, Miljevic, Branka, Crilley, Leigh R., Surawski, Nicholas C., Bartsch, Jennifer, Salimi, Farhad, Uhde, Erik, Schnelle-Kreis, Jürgen, Orasche, Jürgen, Ristovski, Zoran, Ayoko, Godwin A., Zimmermann, Ralf, & Morawska, Lidia (2016) Characterisation of the impact of open biomass burning on urban air quality in Brisbane, Australia. Environment International, 91, pp. 230-242.

Direitos

Copyright 2016 Elsevier

Licensed under the Creative Commons Attribution; Non-Commercial; No-Derivatives 4.0 International. DOI: 10.1016/j.envint.2016.02.030

Fonte

School of Chemistry, Physics & Mechanical Engineering; Institute of Health and Biomedical Innovation; Science & Engineering Faculty; School of Advertising, Marketing & Public Relations

Palavras-Chave #040101 Atmospheric Aerosols #050206 Environmental Monitoring #090799 Environmental Engineering not elsewhere classified #bushfire #wildfire #aerosol #particle #air pollutant #aerosol mass spectrometry
Tipo

Journal Article